Catalytic wet air oxidation of acetic acid over different ruthenium catalysts

Ruthenium catalysts were prepared by impregnation of different supports: ZrO 2, CeO 2, TiO 2, ZrO 2–CeO 2 and TiO 2–CeO 2. Their activities for acetic acid oxidation in aqueous solution were investigated in a stirred reactor at a reaction temperature of 200 °C and total pressure of 4 MPa. The order...

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Published in	Catalysis communications Vol. 9; no. 13; pp. 2163 - 2167
Main Authors	Wang, Jianbing, Zhu, Wanpeng, He, Xuwen, Yang, Shaoxia
Format	Journal Article
Language	English
Published	Elsevier B.V 20.07.2008
Subjects	Acetic acid Catalytic wet air oxidation Non-lattice oxygen Ruthenium catalyst Ruthenium catalyst Catalytic wet air oxidation Non-lattice oxygen Acetic acid
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ISSN	1566-7367 1873-3905
DOI	10.1016/j.catcom.2008.04.019

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Abstract	Ruthenium catalysts were prepared by impregnation of different supports: ZrO 2, CeO 2, TiO 2, ZrO 2–CeO 2 and TiO 2–CeO 2. Their activities for acetic acid oxidation in aqueous solution were investigated in a stirred reactor at a reaction temperature of 200 °C and total pressure of 4 MPa. The order of the catalyst activity obtained was RuO 2/ZrO 2–CeO 2 > RuO 2/CeO 2 > RuO 2/TiO 2–CeO 2 > RuO 2/ZrO 2 > RuO 2/TiO 2, which corresponds to surface concentration of non-lattice oxygen (defect-oxide or hydroxyl-like group) of these catalysts. The non-lattice oxygen on the catalyst surface plays an important role in the catalytic activity.
AbstractList	Ruthenium catalysts were prepared by impregnation of different supports: ZrO 2, CeO 2, TiO 2, ZrO 2–CeO 2 and TiO 2–CeO 2. Their activities for acetic acid oxidation in aqueous solution were investigated in a stirred reactor at a reaction temperature of 200 °C and total pressure of 4 MPa. The order of the catalyst activity obtained was RuO 2/ZrO 2–CeO 2 > RuO 2/CeO 2 > RuO 2/TiO 2–CeO 2 > RuO 2/ZrO 2 > RuO 2/TiO 2, which corresponds to surface concentration of non-lattice oxygen (defect-oxide or hydroxyl-like group) of these catalysts. The non-lattice oxygen on the catalyst surface plays an important role in the catalytic activity.
Author	He, Xuwen Wang, Jianbing Zhu, Wanpeng Yang, Shaoxia
Author_xml	– sequence: 1 givenname: Jianbing surname: Wang fullname: Wang, Jianbing email: wang-jb03@mails.tsinghua.edu.cn organization: School of Chemical and Environmental Engineering, Beijing Campus, China University of Mining and Technology, Beijing 100083, China – sequence: 2 givenname: Wanpeng surname: Zhu fullname: Zhu, Wanpeng organization: Department of Environmental Science and Engineering, Tsinghua University, Beijing 100084, China – sequence: 3 givenname: Xuwen surname: He fullname: He, Xuwen organization: School of Chemical and Environmental Engineering, Beijing Campus, China University of Mining and Technology, Beijing 100083, China – sequence: 4 givenname: Shaoxia surname: Yang fullname: Yang, Shaoxia organization: Department of Environmental Science and Engineering, Tsinghua University, Beijing 100084, China
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SubjectTerms	Acetic acid Catalytic wet air oxidation Non-lattice oxygen Ruthenium catalyst
Title	Catalytic wet air oxidation of acetic acid over different ruthenium catalysts
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