Simultaneous enhancement in charge separation and interfacial charge transfer of BiVO4 photoanode for photoelectrochemical water oxidation
1A facile method for preparing Cu(I) vanadate-BiVO4 p-n heterojuction photoanode.2Role of Cu(I) vanadate in improving the kinetics of charge transport was uncovered.3Efficient interfacial charge transfer and high photostability was achieved. Bismuth vanadate (BiVO4) has been identified as one of the...
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| Published in | Journal of the Taiwan Institute of Chemical Engineers Vol. 111; pp. 80 - 89 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.06.2020
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1876-1070 1876-1089 |
| DOI | 10.1016/j.jtice.2020.05.012 |
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| Abstract | 1A facile method for preparing Cu(I) vanadate-BiVO4 p-n heterojuction photoanode.2Role of Cu(I) vanadate in improving the kinetics of charge transport was uncovered.3Efficient interfacial charge transfer and high photostability was achieved.
Bismuth vanadate (BiVO4) has been identified as one of the promising photoanode materials for photoelectrochemical (PEC) water splitting. Nevertheless, the serious charge recombination and sluggish kinetics of oxygen evolution reaction (OER) are the main factors limiting its PEC performance. In this contribution, copper incorporated nanostructured BiVO4 photoanodes (nanoCu:BiVO4) were prepared by converting the electrodeposited BiOI nanosheets in the presence of copper and vanadium sources and subsequent thermal treatment. nanoCu:BiVO4 prepared with a suitable amount of copper consists of well-interconnected BiVO4 nanoparticles coated with p-type Cu(I) vanadate. The well-interconnected structure improved the kinetics of the charge transport, whereas n–p heterojunction formed between BiVO4 and Cu(I) vanadate remarkably improved the efficiencies of charge separation and interfacial charge transfer. Further improvement in OER kinetics and photostability of nanoCu:BiVO4 was demonstrated by interfacing nanoCu:BiVO4 with nickel-iron oxyhydroxide based OER catalyst. |
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| AbstractList | 1A facile method for preparing Cu(I) vanadate-BiVO4 p-n heterojuction photoanode.2Role of Cu(I) vanadate in improving the kinetics of charge transport was uncovered.3Efficient interfacial charge transfer and high photostability was achieved.
Bismuth vanadate (BiVO4) has been identified as one of the promising photoanode materials for photoelectrochemical (PEC) water splitting. Nevertheless, the serious charge recombination and sluggish kinetics of oxygen evolution reaction (OER) are the main factors limiting its PEC performance. In this contribution, copper incorporated nanostructured BiVO4 photoanodes (nanoCu:BiVO4) were prepared by converting the electrodeposited BiOI nanosheets in the presence of copper and vanadium sources and subsequent thermal treatment. nanoCu:BiVO4 prepared with a suitable amount of copper consists of well-interconnected BiVO4 nanoparticles coated with p-type Cu(I) vanadate. The well-interconnected structure improved the kinetics of the charge transport, whereas n–p heterojunction formed between BiVO4 and Cu(I) vanadate remarkably improved the efficiencies of charge separation and interfacial charge transfer. Further improvement in OER kinetics and photostability of nanoCu:BiVO4 was demonstrated by interfacing nanoCu:BiVO4 with nickel-iron oxyhydroxide based OER catalyst. |
| Author | Lin, Chia-Yu Chueh, Yu-Chien Ko, Ting-Rong Lai, Yi-Hsuan |
| Author_xml | – sequence: 1 givenname: Ting-Rong surname: Ko fullname: Ko, Ting-Rong organization: Department of Materials and Optoelectronic Science, National Sun Yat-sen University, No. 70, Lienhai Road, Kaohsiung 80424, Taiwan – sequence: 2 givenname: Yu-Chien surname: Chueh fullname: Chueh, Yu-Chien organization: Department of Chemical Engineering, National Cheng Kung University, No. 1, University Road, Tainan 70101, Taiwan – sequence: 3 givenname: Yi-Hsuan surname: Lai fullname: Lai, Yi-Hsuan email: yhlai@gs.ncku.edu.tw organization: Department of Materials Science and Engineering, National Cheng Kung University, No. 1, University Road, Tainan 70101, Taiwan – sequence: 4 givenname: Chia-Yu surname: Lin fullname: Lin, Chia-Yu email: cyl44@mail.ncku.edu.tw organization: Department of Chemical Engineering, National Cheng Kung University, No. 1, University Road, Tainan 70101, Taiwan |
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| Keywords | Photoelectrochemistry Bismuth vanadate Nickel-iron oxyhydroxide-borate Water oxidation Heterojunction |
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| Title | Simultaneous enhancement in charge separation and interfacial charge transfer of BiVO4 photoanode for photoelectrochemical water oxidation |
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