GRANADA: A Generic RAdiative traNsfer AnD non-LTE population algorithm

We present in this paper the Generic RAdiative traNsfer AnD non-LTE population Algorithm (GRANADA). This model is able to compute non-LTE populations for vibrational, rotational, spin (i.e., NO and OH), and electronic (i.e., O2) states in a given planetary atmosphere. The model is very flexible and...

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Published in	Journal of quantitative spectroscopy & radiative transfer Vol. 113; no. 14; pp. 1771 - 1817
Main Authors	Funke, B., López-Puertas, M., García-Comas, M., Kaufmann, M., Höpfner, M., Stiller, G.P.
Format	Journal Article
Language	English
Published	Elsevier Ltd 01.09.2012
Subjects	CH4 Climatology CO2 Earth's atmosphere H2O HCN HNO3 Infrared emissions N2O NO2 Non-LTE Climatology NO O2 H2O O3 N2 CO2 Earth's atmosphere N2O HNO3 CO Non-LTE CH4 NO2 HCN Infrared emissions OH
Online Access	Get full text
ISSN	0022-4073 1879-1352
DOI	10.1016/j.jqsrt.2012.05.001

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Abstract	We present in this paper the Generic RAdiative traNsfer AnD non-LTE population Algorithm (GRANADA). This model is able to compute non-LTE populations for vibrational, rotational, spin (i.e., NO and OH), and electronic (i.e., O2) states in a given planetary atmosphere. The model is very flexible and can be used for computing very accurate non-LTE populations or for calculating reasonably accurate but at high speed non-LTE populations in order to implement it into non-LTE remote sensing retrievals. We describe the model in detail and present an update of the non-LTE collisional processes and their rate coefficients for the most important molecules in Earth's atmosphere. In addition, we have applied the model to the most important atmospheric infrared emitters including 13 species (H2O, CO2, O3, N2O, CO, CH4, O2, NO, NO2, HNO3, OH, N2, and HCN) and 460 excited vibrational or electronic energy levels. Non-LTE populations for all these energy levels have been calculated for 48 reference atmospheres expanding from the surface up to 200km, including seasonal (January, April, July and October), latitudinal (75°S, 45°S, 10°S, 10°N, 45°N, 75°N) and diurnal (day and night) coverages. The effects of the most recent updates of the non-LTE collisional parameters on the non-LTE populations are briefly described. This climatology is available online to the community and it can be used for estimating non-LTE effects at specific conditions and for testing and validation studies. ► We present the Generic RAdiative traNsfer AnD non-LTE population Algorithm (GRANADA). ► It computes vibration/rotation/spin/electronic populations of planetary atmospheres. ► We update the non-LTE collisional processes and rates for the atmospheric molecules. ► We present a non-LTE climatology for H2O, CO2, O3, N2O, CO, CH4, O2, NO, NO2, HNO3, OH, N2 and HCN.
AbstractList	We present in this paper the Generic RAdiative traNsfer AnD non-LTE population Algorithm (GRANADA). This model is able to compute non-LTE populations for vibrational, rotational, spin (i.e., NO and OH), and electronic (i.e., O2) states in a given planetary atmosphere. The model is very flexible and can be used for computing very accurate non-LTE populations or for calculating reasonably accurate but at high speed non-LTE populations in order to implement it into non-LTE remote sensing retrievals. We describe the model in detail and present an update of the non-LTE collisional processes and their rate coefficients for the most important molecules in Earth's atmosphere. In addition, we have applied the model to the most important atmospheric infrared emitters including 13 species (H2O, CO2, O3, N2O, CO, CH4, O2, NO, NO2, HNO3, OH, N2, and HCN) and 460 excited vibrational or electronic energy levels. Non-LTE populations for all these energy levels have been calculated for 48 reference atmospheres expanding from the surface up to 200km, including seasonal (January, April, July and October), latitudinal (75°S, 45°S, 10°S, 10°N, 45°N, 75°N) and diurnal (day and night) coverages. The effects of the most recent updates of the non-LTE collisional parameters on the non-LTE populations are briefly described. This climatology is available online to the community and it can be used for estimating non-LTE effects at specific conditions and for testing and validation studies. ► We present the Generic RAdiative traNsfer AnD non-LTE population Algorithm (GRANADA). ► It computes vibration/rotation/spin/electronic populations of planetary atmospheres. ► We update the non-LTE collisional processes and rates for the atmospheric molecules. ► We present a non-LTE climatology for H2O, CO2, O3, N2O, CO, CH4, O2, NO, NO2, HNO3, OH, N2 and HCN.
Author	Höpfner, M. López-Puertas, M. Kaufmann, M. García-Comas, M. Stiller, G.P. Funke, B.
Author_xml	– sequence: 1 givenname: B. surname: Funke fullname: Funke, B. organization: Instituto de Astrofísica de Andalucía, CSIC, Apdo. 3004, 18008 Granada, Spain – sequence: 2 givenname: M. surname: López-Puertas fullname: López-Puertas, M. email: puertas@iaa.es organization: Instituto de Astrofísica de Andalucía, CSIC, Apdo. 3004, 18008 Granada, Spain – sequence: 3 givenname: M. surname: García-Comas fullname: García-Comas, M. organization: Instituto de Astrofísica de Andalucía, CSIC, Apdo. 3004, 18008 Granada, Spain – sequence: 4 givenname: M. surname: Kaufmann fullname: Kaufmann, M. organization: Institute of Energy and Climate Research - Stratosphere, Forschungszentrum Jülich GmbH, 52425 Jülich, Germany – sequence: 5 givenname: M. surname: Höpfner fullname: Höpfner, M. organization: Karlsruhe Institute of Technology, Institute for Meteorology and Climate Research, Postfach 3640, 76021 Karlsruhe, Germany – sequence: 6 givenname: G.P. surname: Stiller fullname: Stiller, G.P. organization: Karlsruhe Institute of Technology, Institute for Meteorology and Climate Research, Postfach 3640, 76021 Karlsruhe, Germany
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Keywords	Climatology NO O2 H2O O3 N2 CO2 Earth's atmosphere N2O HNO3 CO Non-LTE CH4 NO2 HCN Infrared emissions OH
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Snippet	We present in this paper the Generic RAdiative traNsfer AnD non-LTE population Algorithm (GRANADA). This model is able to compute non-LTE populations for...
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SubjectTerms	CH4 Climatology CO2 Earth's atmosphere H2O HCN HNO3 Infrared emissions N2O NO2 Non-LTE
Title	GRANADA: A Generic RAdiative traNsfer AnD non-LTE population algorithm
URI	https://dx.doi.org/10.1016/j.jqsrt.2012.05.001
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