Blue, green, and red full-color ultralong afterglow in nitrogen-doped carbon dots
Carbon dots (CDs) with tunable emission colors and multiple emission modes are highly desirable in advanced optical anti-counterfeiting. Some pioneering efforts to trigger additional long-lived emission modes, nevertheless, did not perfectly solve the issue of printability and color-tunability in pr...
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| Published in | Nanoscale Vol. 11; no. 14; pp. 6584 - 6590 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Royal Society of Chemistry
04.04.2019
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| Subjects | |
| Online Access | Get full text |
| ISSN | 2040-3364 2040-3372 2040-3372 |
| DOI | 10.1039/C8NR09672D |
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| Abstract | Carbon dots (CDs) with tunable emission colors and multiple emission modes are highly desirable in advanced optical anti-counterfeiting. Some pioneering efforts to trigger additional long-lived emission modes, nevertheless, did not perfectly solve the issue of printability and color-tunability in practical applications. Herein, we developed an encapsulating-dissolving-recrystallization route for the synthesis of CD-based anti-counterfeiting inks, and accordingly realized blue, green, and red full-color afterglow emissions from these CD-based inks when printed on paper. The printed inks simultaneously possessed triple emission modes including fluorescence (FL), delayed fluorescence (DF), and room-temperature phosphorescence (RTP), among which the long-lived emissions (DF and RTP) could be selectively activated by using different excitation wavelengths. We believe that the proposed synthetic route in this work may promote the development of multicolor-encoded and multiple-mode-integrated optical anti-counterfeiting systems, and will expand the application of CD-based materials to the fields of sensing, photodynamic therapy and bio-imaging. |
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| AbstractList | Carbon dots (CDs) with tunable emission colors and multiple emission modes are highly desirable in advanced optical anti-counterfeiting. Some pioneering efforts to trigger additional long-lived emission modes, nevertheless, did not perfectly solve the issue of printability and color-tunability in practical applications. Herein, we developed an encapsulating-dissolving-recrystallization route for the synthesis of CD-based anti-counterfeiting inks, and accordingly realized blue, green, and red full-color afterglow emissions from these CD-based inks when printed on paper. The printed inks simultaneously possessed triple emission modes including fluorescence (FL), delayed fluorescence (DF), and room-temperature phosphorescence (RTP), among which the long-lived emissions (DF and RTP) could be selectively activated by using different excitation wavelengths. We believe that the proposed synthetic route in this work may promote the development of multicolor-encoded and multiple-mode-integrated optical anti-counterfeiting systems, and will expand the application of CD-based materials to the fields of sensing, photodynamic therapy and bio-imaging. Carbon dots (CDs) with tunable emission colors and multiple emission modes are highly desirable in advanced optical anti-counterfeiting. Some pioneering efforts to trigger additional long-lived emission modes, nevertheless, did not perfectly solve the issue of printability and color-tunability in practical applications. Herein, we developed an encapsulating-dissolving-recrystallization route for the synthesis of CD-based anti-counterfeiting inks, and accordingly realized blue, green, and red full-color afterglow emissions from these CD-based inks when printed on paper. The printed inks simultaneously possessed triple emission modes including fluorescence (FL), delayed fluorescence (DF), and room-temperature phosphorescence (RTP), among which the long-lived emissions (DF and RTP) could be selectively activated by using different excitation wavelengths. We believe that the proposed synthetic route in this work may promote the development of multicolor-encoded and multiple-mode-integrated optical anti-counterfeiting systems, and will expand the application of CD-based materials to the fields of sensing, photodynamic therapy and bio-imaging.Carbon dots (CDs) with tunable emission colors and multiple emission modes are highly desirable in advanced optical anti-counterfeiting. Some pioneering efforts to trigger additional long-lived emission modes, nevertheless, did not perfectly solve the issue of printability and color-tunability in practical applications. Herein, we developed an encapsulating-dissolving-recrystallization route for the synthesis of CD-based anti-counterfeiting inks, and accordingly realized blue, green, and red full-color afterglow emissions from these CD-based inks when printed on paper. The printed inks simultaneously possessed triple emission modes including fluorescence (FL), delayed fluorescence (DF), and room-temperature phosphorescence (RTP), among which the long-lived emissions (DF and RTP) could be selectively activated by using different excitation wavelengths. We believe that the proposed synthetic route in this work may promote the development of multicolor-encoded and multiple-mode-integrated optical anti-counterfeiting systems, and will expand the application of CD-based materials to the fields of sensing, photodynamic therapy and bio-imaging. |
| Author | Zhou, Tian-Liang Zhuang, Yixi Lin, Cunjian Xie, Rong-Jun Li, Wuhui |
| Author_xml | – sequence: 1 givenname: Cunjian surname: Lin fullname: Lin, Cunjian organization: College of Materials, Xiamen University, Xiamen, 361005 P.R. China – sequence: 2 givenname: Yixi orcidid: 0000-0001-7290-1033 surname: Zhuang fullname: Zhuang, Yixi organization: College of Materials, Xiamen University, Xiamen, 361005 P.R. China – sequence: 3 givenname: Wuhui surname: Li fullname: Li, Wuhui organization: College of Materials, Xiamen University, Xiamen, 361005 P.R. China – sequence: 4 givenname: Tian-Liang surname: Zhou fullname: Zhou, Tian-Liang organization: College of Materials, Xiamen University, Xiamen, 361005 P.R. China – sequence: 5 givenname: Rong-Jun orcidid: 0000-0002-8387-1316 surname: Xie fullname: Xie, Rong-Jun organization: College of Materials, Xiamen University, Xiamen, 361005 P.R. China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30601528$$D View this record in MEDLINE/PubMed |
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| Snippet | Carbon dots (CDs) with tunable emission colors and multiple emission modes are highly desirable in advanced optical anti-counterfeiting. Some pioneering... |
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| SubjectTerms | Carbon dots Coding Color Counterfeiting Excitation spectra Fluorescence Fourier transforms Image transmission Infrared spectra Inks Phosphorescence Photodynamic therapy Photoelectrons Recrystallization Spectrum analysis Synthesis Transmission electron microscopy Ultraviolet radiation Wavelengths |
| Title | Blue, green, and red full-color ultralong afterglow in nitrogen-doped carbon dots |
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