Two-phase flow and mass transfer in microchannels: A review from local mechanism to global models

•The hydrodynamics, mixing and mass transfer of two-phase processes are reviewed.•Bubble/droplet formation mechanism and scaling models are summarized.•The dynamic behavior during formation stage is highlighted.•The circulation topology and mixing inside both droplets and slugs are discussed.•The in...

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Published inChemical engineering science Vol. 229; p. 116017
Main Authors Yao, Chaoqun, Zhao, Yuchao, Ma, Haiyun, Liu, Yanyan, Zhao, Qiankun, Chen, Guangwen
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 16.01.2021
Subjects
Microfluidic
Microreactor
Multiphase
Transport
Viscous fluid
Microreactor
Transport
Multiphase
Viscous fluid
Microfluidic
Online AccessGet full text
ISSN0009-2509
1873-4405
DOI10.1016/j.ces.2020.116017

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Abstract •The hydrodynamics, mixing and mass transfer of two-phase processes are reviewed.•Bubble/droplet formation mechanism and scaling models are summarized.•The dynamic behavior during formation stage is highlighted.•The circulation topology and mixing inside both droplets and slugs are discussed.•The interfacial mass transfer regimes and simulative models are presented. Microreaction technology is preferential in process intensification and chemical synthesis, especially in multiphase applications. A thorough understanding of the hydrodynamics and mass transfer is the pre-requisite for implementing such applications. This review discusses the recent progress on the flow and mass transfer of two-phase systems in microchannels, in a multi-scale view from local mechanism to global behavior. The flow patterns, the formation of bubbles/droplets, and the manipulation of bubbles/droplets are presented and discussed in detail. The mass transfer aspects include the velocity profile and mixing inside droplets/slugs, as well as the interfacial mass transfer mechanism and simulative models. The aim of the review is to show directly the physical ingredients which determine the transport phenomena, help explain the observed behavior, and guide reactor design. To simplify the physical ingredients, the attention is focused on straight channels while phenomena in other channels (e.g., meandering channel) are neglected.
AbstractList •The hydrodynamics, mixing and mass transfer of two-phase processes are reviewed.•Bubble/droplet formation mechanism and scaling models are summarized.•The dynamic behavior during formation stage is highlighted.•The circulation topology and mixing inside both droplets and slugs are discussed.•The interfacial mass transfer regimes and simulative models are presented. Microreaction technology is preferential in process intensification and chemical synthesis, especially in multiphase applications. A thorough understanding of the hydrodynamics and mass transfer is the pre-requisite for implementing such applications. This review discusses the recent progress on the flow and mass transfer of two-phase systems in microchannels, in a multi-scale view from local mechanism to global behavior. The flow patterns, the formation of bubbles/droplets, and the manipulation of bubbles/droplets are presented and discussed in detail. The mass transfer aspects include the velocity profile and mixing inside droplets/slugs, as well as the interfacial mass transfer mechanism and simulative models. The aim of the review is to show directly the physical ingredients which determine the transport phenomena, help explain the observed behavior, and guide reactor design. To simplify the physical ingredients, the attention is focused on straight channels while phenomena in other channels (e.g., meandering channel) are neglected.
ArticleNumber 116017
Author Zhao, Yuchao
Yao, Chaoqun
Zhao, Qiankun
Liu, Yanyan
Chen, Guangwen
Ma, Haiyun
Author_xml – sequence: 1
  givenname: Chaoqun
  surname: Yao
  fullname: Yao, Chaoqun
  organization: Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China
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  givenname: Yuchao
  orcidid: 0000-0001-7238-7265
  surname: Zhao
  fullname: Zhao, Yuchao
  organization: Shandong Collaborative Innovation Center of Light Hydrocarbon Transformation and Utilization, College of Chemistry & Chemical Engineering, Yantai University, Yantai 264005, China
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  givenname: Haiyun
  surname: Ma
  fullname: Ma, Haiyun
  organization: Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China
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  givenname: Yanyan
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  fullname: Liu, Yanyan
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  givenname: Guangwen
  orcidid: 0000-0001-5290-7921
  surname: Chen
  fullname: Chen, Guangwen
  email: gwchen@dicp.ac.cn
  organization: Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China
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Viscous fluid
Title Two-phase flow and mass transfer in microchannels: A review from local mechanism to global models
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