Leaching of vanadium and chromium from converter vanadium slag intensified with surface wettability
Technology intensified with surface wettability was introduced to leach vanadium and chromium from converter vanadium slag without roasting. Parameters affecting the leaching efficiency of vanadium and chromium were investigated: sulfuric acid concentration, MnO 2 -to-slag mass ratio, liquid-to-soli...
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| Published in | Journal of Central South University Vol. 25; no. 6; pp. 1317 - 1325 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Changsha
Central South University
01.06.2018
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2095-2899 2227-5223 |
| DOI | 10.1007/s11771-018-3828-2 |
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| Abstract | Technology intensified with surface wettability was introduced to leach vanadium and chromium from converter vanadium slag without roasting. Parameters affecting the leaching efficiency of vanadium and chromium were investigated: sulfuric acid concentration, MnO
2
-to-slag mass ratio, liquid-to-solid ratio, leaching time, leaching temperature, and sodium dodecyl sulfate (SDS)-to-slag mass ratio. The leaching efficiencies of vanadium and chromium were 33.46 % and 20.02 % higher in the presence of MnO
2
and SDS, respectively, compared to the control. The leaching efficiencies of vanadium and chromium were 68.93 % and 30.74 %, respectively, under the optimum conditions: sulfuric acid concentration 40 wt%, MnO
2
-to-slag mass ratio 10.0 wt%, liquid-to-solid ratio 5:1 mL/g; 12 h; 90 °C; and SDS-to-slag mass ratio 0.25 wt%. The analysis of the reaction mechanism in the leaching process indicates that MnO
2
combined with protons (H
+
) could oxidize low-valent vanadium and chromium; SDS could change the chemical behavior and decrease the surface tension of the aqueous solution to favor MnO
2
oxidization. |
|---|---|
| AbstractList | Technology intensified with surface wettability was introduced to leach vanadium and chromium from converter vanadium slag without roasting. Parameters affecting the leaching efficiency of vanadium and chromium were investigated: sulfuric acid concentration, MnO2-to-slag mass ratio, liquid-to-solid ratio, leaching time, leaching temperature, and sodium dodecyl sulfate (SDS)-to-slag mass ratio. The leaching efficiencies of vanadium and chromium were 33.46 % and 20.02 % higher in the presence of MnO2 and SDS, respectively, compared to the control. The leaching efficiencies of vanadium and chromium were 68.93 % and 30.74 %, respectively, under the optimum conditions: sulfuric acid concentration 40 wt%, MnO2-to-slag mass ratio 10.0 wt%, liquid-to-solid ratio 5:1 mL/g; 12 h; 90 °C; and SDS-to-slag mass ratio 0.25 wt%. The analysis of the reaction mechanism in the leaching process indicates that MnO2 combined with protons (H+) could oxidize low-valent vanadium and chromium; SDS could change the chemical behavior and decrease the surface tension of the aqueous solution to favor MnO2 oxidization. Technology intensified with surface wettability was introduced to leach vanadium and chromium from converter vanadium slag without roasting. Parameters affecting the leaching efficiency of vanadium and chromium were investigated: sulfuric acid concentration, MnO 2 -to-slag mass ratio, liquid-to-solid ratio, leaching time, leaching temperature, and sodium dodecyl sulfate (SDS)-to-slag mass ratio. The leaching efficiencies of vanadium and chromium were 33.46 % and 20.02 % higher in the presence of MnO 2 and SDS, respectively, compared to the control. The leaching efficiencies of vanadium and chromium were 68.93 % and 30.74 %, respectively, under the optimum conditions: sulfuric acid concentration 40 wt%, MnO 2 -to-slag mass ratio 10.0 wt%, liquid-to-solid ratio 5:1 mL/g; 12 h; 90 °C; and SDS-to-slag mass ratio 0.25 wt%. The analysis of the reaction mechanism in the leaching process indicates that MnO 2 combined with protons (H + ) could oxidize low-valent vanadium and chromium; SDS could change the chemical behavior and decrease the surface tension of the aqueous solution to favor MnO 2 oxidization. |
| Author | Peng, Hao Liu, Zuo-hua Yang, Qi-wen Xie, Zhao-ming Tao, Chang-yuan |
| Author_xml | – sequence: 1 givenname: Qi-wen surname: Yang fullname: Yang, Qi-wen organization: Chongqing Key Laboratory of Chemical Process for Clean Energy and Resource Utilization, Chongqing University, College of Chemistry and Chemical Engineering, Chongqing University – sequence: 2 givenname: Zhao-ming surname: Xie fullname: Xie, Zhao-ming email: xiezm@cqu.edu.cn organization: Chongqing Key Laboratory of Chemical Process for Clean Energy and Resource Utilization, Chongqing University, College of Chemistry and Chemical Engineering, Chongqing University – sequence: 3 givenname: Hao surname: Peng fullname: Peng, Hao organization: Chongqing Key Laboratory of Chemical Process for Clean Energy and Resource Utilization, Chongqing University, College of Chemistry and Chemical Engineering, Chongqing University – sequence: 4 givenname: Zuo-hua surname: Liu fullname: Liu, Zuo-hua email: liuzuohua@cqu.edu.cn organization: Chongqing Key Laboratory of Chemical Process for Clean Energy and Resource Utilization, Chongqing University, College of Chemistry and Chemical Engineering, Chongqing University – sequence: 5 givenname: Chang-yuan surname: Tao fullname: Tao, Chang-yuan organization: Chongqing Key Laboratory of Chemical Process for Clean Energy and Resource Utilization, Chongqing University, College of Chemistry and Chemical Engineering, Chongqing University |
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| Keywords | 二氧化锰 chromium 钒 十二烷基硫酸钠 vanadium leaching 铬 surfactant MnO 浸出 |
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| Snippet | Technology intensified with surface wettability was introduced to leach vanadium and chromium from converter vanadium slag without roasting. Parameters... |
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| SubjectTerms | Chromium Engineering Leaching Manganese dioxide Metallic Materials Organic chemistry Reaction mechanisms Sodium dodecyl sulfate Steel converters Sulfuric acid Surface tension Vanadium Wettability |
| Title | Leaching of vanadium and chromium from converter vanadium slag intensified with surface wettability |
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