Spectroscopic investigations of thulium doped YAG and YAP crystals between 77 K and 300 K for short-wavelength infrared lasers
We present detailed measurements of laser relevant cross sections of thulium doped yttrium-aluminum-garnet (Tm:YAG) and yttrium-aluminum-perovskite (Tm:YAP), including the absorption cross sections for the H63 to H43 transition near 800 nm, and the absorption and emission cross sections for the tran...
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| Published in | Journal of luminescence Vol. 202; pp. 427 - 437 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.10.2018
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0022-2313 1872-7883 |
| DOI | 10.1016/j.jlumin.2018.05.070 |
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| Abstract | We present detailed measurements of laser relevant cross sections of thulium doped yttrium-aluminum-garnet (Tm:YAG) and yttrium-aluminum-perovskite (Tm:YAP), including the absorption cross sections for the H63 to H43 transition near 800 nm, and the absorption and emission cross sections for the transitions between the H63 and F43 manifolds in the short-wavelength infrared region. For Tm:YAP we present data for all polarization axes. The measurements were carried out at temperatures ranging from 80 K to 300 K. Furthermore, re-absorption free fluorescence lifetimes of the F43 to H63 transition at 77 K, 200 K and 295 K were obtained using the pinhole method. We observed a significant enhancement of the fluorescence lifetime when cooling from room temperature to 77 K. The lifetime was increased from 9.42 ms to 15.22 ms in Tm:YAG and from 3.81 ms to 4.93 ms in Tm:YAP. This indicates that lifetime quenching is present at room temperature, which can be overcome, at least partially, by cryogenic cooling. These data are presented with the scope to qualify these materials for their use in a new generation of cryogenically cooled, short-wavelength infrared, high-energy class diode pumped solid state lasers utilizing the cross relaxation mechanism for pumping. |
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| AbstractList | We present detailed measurements of laser relevant cross sections of thulium doped yttrium-aluminum-garnet (Tm:YAG) and yttrium-aluminum-perovskite (Tm:YAP), including the absorption cross sections for the H63 to H43 transition near 800 nm, and the absorption and emission cross sections for the transitions between the H63 and F43 manifolds in the short-wavelength infrared region. For Tm:YAP we present data for all polarization axes. The measurements were carried out at temperatures ranging from 80 K to 300 K. Furthermore, re-absorption free fluorescence lifetimes of the F43 to H63 transition at 77 K, 200 K and 295 K were obtained using the pinhole method. We observed a significant enhancement of the fluorescence lifetime when cooling from room temperature to 77 K. The lifetime was increased from 9.42 ms to 15.22 ms in Tm:YAG and from 3.81 ms to 4.93 ms in Tm:YAP. This indicates that lifetime quenching is present at room temperature, which can be overcome, at least partially, by cryogenic cooling. These data are presented with the scope to qualify these materials for their use in a new generation of cryogenically cooled, short-wavelength infrared, high-energy class diode pumped solid state lasers utilizing the cross relaxation mechanism for pumping. |
| Author | Uschmann, Ingo Lühder, Tilman Marschner, Heike Lucianetti, Antonio Jambunathan, Venkatesan Mocek, Tomáš Körner, Jörg Reiter, Jürgen Hein, Joachim Kaluza, Malte C. |
| Author_xml | – sequence: 1 givenname: Jörg surname: Körner fullname: Körner, Jörg email: joerg.koerner@uni-jena.de organization: Institute of Optics and Quantum Electronics, Friedrich-Schiller University, Max-Wien Platz 1, 07743 Jena, Germany – sequence: 2 givenname: Tilman surname: Lühder fullname: Lühder, Tilman organization: Institute of Optics and Quantum Electronics, Friedrich-Schiller University, Max-Wien Platz 1, 07743 Jena, Germany – sequence: 3 givenname: Jürgen surname: Reiter fullname: Reiter, Jürgen organization: Institute of Optics and Quantum Electronics, Friedrich-Schiller University, Max-Wien Platz 1, 07743 Jena, Germany – sequence: 4 givenname: Ingo surname: Uschmann fullname: Uschmann, Ingo organization: Institute of Optics and Quantum Electronics, Friedrich-Schiller University, Max-Wien Platz 1, 07743 Jena, Germany – sequence: 5 givenname: Heike surname: Marschner fullname: Marschner, Heike organization: Institute of Optics and Quantum Electronics, Friedrich-Schiller University, Max-Wien Platz 1, 07743 Jena, Germany – sequence: 6 givenname: Venkatesan surname: Jambunathan fullname: Jambunathan, Venkatesan organization: HiLASE Centre, Institute of Physics of the Czech Academy of Sciences, Za Radnicí 828, 252 41 Dolní Břežany, Czech Republic – sequence: 7 givenname: Antonio surname: Lucianetti fullname: Lucianetti, Antonio organization: HiLASE Centre, Institute of Physics of the Czech Academy of Sciences, Za Radnicí 828, 252 41 Dolní Břežany, Czech Republic – sequence: 8 givenname: Tomáš surname: Mocek fullname: Mocek, Tomáš organization: HiLASE Centre, Institute of Physics of the Czech Academy of Sciences, Za Radnicí 828, 252 41 Dolní Břežany, Czech Republic – sequence: 9 givenname: Joachim surname: Hein fullname: Hein, Joachim organization: Institute of Optics and Quantum Electronics, Friedrich-Schiller University, Max-Wien Platz 1, 07743 Jena, Germany – sequence: 10 givenname: Malte C. surname: Kaluza fullname: Kaluza, Malte C. organization: Institute of Optics and Quantum Electronics, Friedrich-Schiller University, Max-Wien Platz 1, 07743 Jena, Germany |
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| Cites_doi | 10.1364/AO.29.001281 10.1364/OL.32.001908 10.1109/3.161321 10.1002/pssa.2210190129 10.1103/PhysRev.136.A954 10.1007/s00340-013-5650-8 10.1364/JOSAB.29.002493 10.1023/B:JAPS.0000032875.04400.a0 10.1103/PhysRevB.40.9464 10.1364/AO.37.004933 10.1364/ASSL.2002.TuB15 10.1364/AO.49.006236 10.1364/JOSAB.23.001770 10.5772/39538 10.1049/el:20030447 10.1117/12.2267881 10.1364/OL.37.004546 10.1109/3.502365 |
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| Keywords | Thulium YALO Cross section Cryogenic cooling YAP Spectra Fluorescence lifetime Short-wavelength infrared lasers YAG |
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| SubjectTerms | Cross section Cryogenic cooling Fluorescence lifetime Short-wavelength infrared lasers Spectra Thulium YAG YALO YAP |
| Title | Spectroscopic investigations of thulium doped YAG and YAP crystals between 77 K and 300 K for short-wavelength infrared lasers |
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