Synergistic effect of blended primary and secondary amines functionalized onto the silica on CO2 capture performance
Amine-functionalized silica sorbents were synthesized by blending (3-aminopropyl)trimethoxysilane (1NSP) and [3-(methylamino)propyl]trimethoxysilane (1NS-S) of varying proportions and incorporating it in the support via incipient wetness technique. Adsorption characteristics were examined at a desig...
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| Published in | The Korean journal of chemical engineering Vol. 36; no. 8; pp. 1267 - 1273 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Springer US
01.08.2019
Springer Nature B.V 한국화학공학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0256-1115 1975-7220 |
| DOI | 10.1007/s11814-019-0321-z |
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| Abstract | Amine-functionalized silica sorbents were synthesized by blending (3-aminopropyl)trimethoxysilane (1NSP) and [3-(methylamino)propyl]trimethoxysilane (1NS-S) of varying proportions and incorporating it in the support via incipient wetness technique. Adsorption characteristics were examined at a design adsorption temperature of 30 oC. The blended amine adsorbents exhibited higher CO
2
adsorption capacity (5.6-6.4 wt%) and CO
2
/N efficiency (0.47-0.48) than 1NS-P and 1NS-S. Among the blended amine adsorbents synthesized in this work, 1NS-PS-50, which has 50% primary amine and 50% secondary amine, is the most ideal for post-combustion CO
2
capture application because it has high CO
2
adsorption capacity, high CO
2
/N efficiency, and better performance than its diamine counterpart, N-[3-(trimethoxysilyl)propyl]ethylenediamine. |
|---|---|
| AbstractList | Amine-functionalized silica sorbents were synthesized by blending (3-aminopropyl)trimethoxysilane (1NSP) and [3-(methylamino)propyl]trimethoxysilane (1NS-S) of varying proportions and incorporating it in the support via incipient wetness technique. Adsorption characteristics were examined at a design adsorption temperature of 30 oC. The blended amine adsorbents exhibited higher CO2 adsorption capacity (5.6-6.4 wt%) and CO2/N efficiency (0.47-0.48) than 1NS-P and 1NS-S. Among the blended amine adsorbents synthesized in this work, 1NS-PS-50, which has 50% primary amine and 50% secondary amine, is the most ideal for post-combustion CO2 capture application because it has high CO2 adsorption capacity, high CO2/N efficiency, and better performance than its diamine counterpart, N-[3-(trimethoxysilyl)propyl]ethylenediamine. Amine-functionalized silica sorbents were synthesized by blending (3-aminopropyl)trimethoxysilane (1NSP) and [3-(methylamino)propyl]trimethoxysilane (1NS-S) of varying proportions and incorporating it in the support via incipient wetness technique. Adsorption characteristics were examined at a design adsorption temperature of 30 oC. The blended amine adsorbents exhibited higher CO 2 adsorption capacity (5.6-6.4 wt%) and CO 2 /N efficiency (0.47-0.48) than 1NS-P and 1NS-S. Among the blended amine adsorbents synthesized in this work, 1NS-PS-50, which has 50% primary amine and 50% secondary amine, is the most ideal for post-combustion CO 2 capture application because it has high CO 2 adsorption capacity, high CO 2 /N efficiency, and better performance than its diamine counterpart, N-[3-(trimethoxysilyl)propyl]ethylenediamine. Amine-functionalized silica sorbents were synthesized by blending (3-aminopropyl)trimethoxysilane (1NSP) and [3-(methylamino)propyl]trimethoxysilane (1NS-S) of varying proportions and incorporating it in the support via incipient wetness technique. Adsorption characteristics were examined at a design adsorption temperature of 30 oC. The blended amine adsorbents exhibited higher CO2 adsorption capacity (5.6-6.4 wt%) and CO2/N efficiency (0.47- 0.48) than 1NS-P and 1NS-S. Among the blended amine adsorbents synthesized in this work, 1NS-PS-50, which has 50% primary amine and 50% secondary amine, is the most ideal for post-combustion CO2 capture application because it has high CO2 adsorption capacity, high CO2/N efficiency, and better performance than its diamine counterpart, N- [3-(trimethoxysilyl)propyl]ethylenediamine KCI Citation Count: 8 |
| Author | Pacia, Rose Mardie Manianglung, Clinton Ko, Young Soo |
| Author_xml | – sequence: 1 givenname: Clinton surname: Manianglung fullname: Manianglung, Clinton organization: Department of Chemical Engineering, Kongju National University – sequence: 2 givenname: Rose Mardie surname: Pacia fullname: Pacia, Rose Mardie organization: Department of Chemical Engineering, Kongju National University – sequence: 3 givenname: Young Soo surname: Ko fullname: Ko, Young Soo email: ysko@kongju.ac.kr organization: Department of Chemical Engineering, Kongju National University |
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| CitedBy_id | crossref_primary_10_1007_s11814_020_0483_8 crossref_primary_10_1007_s11814_020_0684_1 crossref_primary_10_1016_j_jcou_2020_101320 crossref_primary_10_1016_j_seppur_2020_117065 crossref_primary_10_1016_j_gce_2020_09_005 crossref_primary_10_1016_j_jiec_2025_02_019 crossref_primary_10_1007_s11814_020_0596_0 crossref_primary_10_1016_j_fuel_2024_130898 crossref_primary_10_1016_j_micromeso_2024_112998 crossref_primary_10_1021_acs_energyfuels_4c02513 crossref_primary_10_1007_s11814_020_0565_7 crossref_primary_10_1021_acs_jpcc_2c08453 |
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| Snippet | Amine-functionalized silica sorbents were synthesized by blending (3-aminopropyl)trimethoxysilane (1NSP) and [3-(methylamino)propyl]trimethoxysilane (1NS-S) of... |
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| SubjectTerms | Adsorbents Adsorption Amines Biotechnology Carbon dioxide Carbon sequestration Catalysis Chemistry Chemistry and Materials Science Ethylenediamine Industrial Chemistry/Chemical Engineering Materials Science Moisture content Reaction Engineering Silicon dioxide Sorbents Synergistic effect Synthesis 화학공학 |
| Title | Synergistic effect of blended primary and secondary amines functionalized onto the silica on CO2 capture performance |
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