Linear low-density polyethylene gasification over highly active Ni/CeO2-ZrO2 catalyst for enhanced hydrogen generation
Steam-gasification of linear low-density polyethylene (LLDPE) waste to hydrogen-rich gas has been studied systematically over nickel (10wt.%) loaded on a variety of supports (Al2O3, CeO2, and CeO2-ZrO2) synthesized using a novel solvent deficient method (SDM). The hydrogen selectivity order of the c...
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| Published in | Journal of industrial and engineering chemistry (Seoul, Korea) Vol. 94; pp. 336 - 342 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
25.02.2021
한국공업화학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1226-086X 1876-794X |
| DOI | 10.1016/j.jiec.2020.11.005 |
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| Abstract | Steam-gasification of linear low-density polyethylene (LLDPE) waste to hydrogen-rich gas has been studied systematically over nickel (10wt.%) loaded on a variety of supports (Al2O3, CeO2, and CeO2-ZrO2) synthesized using a novel solvent deficient method (SDM). The hydrogen selectivity order of the catalysts was reported as Ni/CeO2-ZrO2>Ni/CeO2>Ni/Al2O3. The highest catalytic H2 selectivity of the Ni/CeO2-ZrO2 catalyst was reported to be ∼76vol.%, and was attributed to the smaller nickel crystals that were finely dispersed on the support, and to formation of Ce1-xZrxO2-δ solid solutions. The Ce1-xZrxO2-δ solid solution in the Ni/CeO2-ZrO2 catalyst was observed to be bi-functional, thus reflecting the acceleration of the water gas shift and the oxidation of carbon to CO and CO2. The better resistance of the Ni/CeO2-ZrO2 catalyst towards coke deposition also indicated its potential for commercial-scale applications for the steam gasification of plastics. Therefore, this research provides an advanced route to recycle LLDPE plastic waste into hydrogen fuel, which presents both economical and environmental benefits. |
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| AbstractList | Steam-gasification of linear low-density polyethylene (LLDPE) waste to hydrogen-rich gas has beenstudied systematically over nickel (10 wt.%) loaded on a variety of supports (Al2O3, CeO2, and CeO2-ZrO2)synthesized using a novel solvent deficient method (SDM). The hydrogen selectivity order of the catalystswas reported as Ni/CeO2-ZrO2>Ni/CeO2>Ni/Al2O3. The highest catalytic H2 selectivity of the Ni/CeO2-ZrO2 catalyst was reported to be76 vol.%, and was attributed to the smaller nickel crystals that werefinely dispersed on the support, and to formation of Ce1-xZrxO2-d solid solutions. The Ce1-xZrxO2-d solidsolution in the Ni/CeO2-ZrO2 catalyst was observed to be bi-functional, thus reflecting the acceleration ofthe water gas shift and the oxidation of carbon to CO and CO2. The better resistance of the Ni/CeO2-ZrO2catalyst towards coke deposition also indicated its potential for commercial-scale applications for thesteam gasification of plastics. Therefore, this research provides an advanced route to recycle LLDPE plasticwaste into hydrogen fuel, which presents both economical and environmental benefits. KCI Citation Count: 18 Steam-gasification of linear low-density polyethylene (LLDPE) waste to hydrogen-rich gas has been studied systematically over nickel (10wt.%) loaded on a variety of supports (Al2O3, CeO2, and CeO2-ZrO2) synthesized using a novel solvent deficient method (SDM). The hydrogen selectivity order of the catalysts was reported as Ni/CeO2-ZrO2>Ni/CeO2>Ni/Al2O3. The highest catalytic H2 selectivity of the Ni/CeO2-ZrO2 catalyst was reported to be ∼76vol.%, and was attributed to the smaller nickel crystals that were finely dispersed on the support, and to formation of Ce1-xZrxO2-δ solid solutions. The Ce1-xZrxO2-δ solid solution in the Ni/CeO2-ZrO2 catalyst was observed to be bi-functional, thus reflecting the acceleration of the water gas shift and the oxidation of carbon to CO and CO2. The better resistance of the Ni/CeO2-ZrO2 catalyst towards coke deposition also indicated its potential for commercial-scale applications for the steam gasification of plastics. Therefore, this research provides an advanced route to recycle LLDPE plastic waste into hydrogen fuel, which presents both economical and environmental benefits. |
| Author | Jang, Seong-Ho Kannapu, Hari Prasad Reddy Park, Young-Kwon Lam, Su Shiung Ahmed, Ashfaq Moogi, Surendar Valizadeh, Soheil Farooq, Abid |
| Author_xml | – sequence: 1 givenname: Abid surname: Farooq fullname: Farooq, Abid organization: School of Environmental Engineering, University of Seoul, Seoul 02504, Republic of Korea – sequence: 2 givenname: Surendar surname: Moogi fullname: Moogi, Surendar organization: School of Environmental Engineering, University of Seoul, Seoul 02504, Republic of Korea – sequence: 3 givenname: Seong-Ho surname: Jang fullname: Jang, Seong-Ho organization: Department of BioEnvironmental Energy, Pusan National University, Miryang 50463, Republic of Korea – sequence: 4 givenname: Hari Prasad Reddy surname: Kannapu fullname: Kannapu, Hari Prasad Reddy organization: School of Environmental Engineering, University of Seoul, Seoul 02504, Republic of Korea – sequence: 5 givenname: Soheil surname: Valizadeh fullname: Valizadeh, Soheil organization: School of Environmental Engineering, University of Seoul, Seoul 02504, Republic of Korea – sequence: 6 givenname: Ashfaq surname: Ahmed fullname: Ahmed, Ashfaq organization: School of Environmental Engineering, University of Seoul, Seoul 02504, Republic of Korea – sequence: 7 givenname: Su Shiung surname: Lam fullname: Lam, Su Shiung organization: Pyrolysis Technology Research Group, Institute of Tropical Aquaculture and Fisheries (Akuatrop), Universiti Malaysia Terengganu, 21030 Kuala Nerus, Terengganu, Malaysia – sequence: 8 givenname: Young-Kwon surname: Park fullname: Park, Young-Kwon email: catalica@uos.ac.kr organization: School of Environmental Engineering, University of Seoul, Seoul 02504, Republic of Korea |
| BackLink | https://www.kci.go.kr/kciportal/ci/sereArticleSearch/ciSereArtiView.kci?sereArticleSearchBean.artiId=ART002686586$$DAccess content in National Research Foundation of Korea (NRF) |
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| Keywords | Ni/CeO2-ZrO2 catalyst LLDPE Solid solution Hydrogen Steam gasification |
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| Title | Linear low-density polyethylene gasification over highly active Ni/CeO2-ZrO2 catalyst for enhanced hydrogen generation |
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