Construction of dye-sensitized solar cells using wet chemical route synthesized MoSe2 counter electrode
[Display omitted] •Wet chemical methodology was used to synthesize MoSe2 as a CE for DSSCs.•High PCE of 7.28% achieves using MoSe2 CE, equivalent to Pt CE (7.40%).•Uniform morphology with active sites promotes electrocatalytic activity. This paper presents a simple and large area wet chemical prepar...
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| Published in | Journal of industrial and engineering chemistry (Seoul, Korea) Vol. 69; pp. 379 - 386 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
25.01.2019
한국공업화학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1226-086X 1876-794X |
| DOI | 10.1016/j.jiec.2018.10.001 |
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| Abstract | [Display omitted]
•Wet chemical methodology was used to synthesize MoSe2 as a CE for DSSCs.•High PCE of 7.28% achieves using MoSe2 CE, equivalent to Pt CE (7.40%).•Uniform morphology with active sites promotes electrocatalytic activity.
This paper presents a simple and large area wet chemical preparation route for molybdenum diselenide (MoSe2) atomic layers. MoSe2 was synthesized onto fluorine doped tin oxide substrates and could be directly used as a counter electrode (CE) for dye-sensitized solar cells (DSSCs). The role of deposition time on the growth of MoSe2 CE was elaborately discussed using Raman, X-ray diffraction and photoluminescence studies. Influence of wet chemical growth time on the surface modification of MoSe2 CE was evidently demonstrated by scanning electron microscopy and atomic force microscopy studies. The MoSe2 CE electrode has lower charge transfer resistance and superior electrocatalytic activity towards triiodide/iodide redox behavior, comparable to conventional Pt CEs. High power conversion efficiency of 7.28% was achieved, equivalent to scarce noble metal Pt CE (7.40%). Uniform surface morphology with active edge sites highly dominated to promote the superior electrocatalytic activity. This work opens a way to use an economical wet chemical method to fabricate the layered MoSe2 CE as a replacement for high cost Pt based CE for DSSCs. |
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| AbstractList | [Display omitted]
•Wet chemical methodology was used to synthesize MoSe2 as a CE for DSSCs.•High PCE of 7.28% achieves using MoSe2 CE, equivalent to Pt CE (7.40%).•Uniform morphology with active sites promotes electrocatalytic activity.
This paper presents a simple and large area wet chemical preparation route for molybdenum diselenide (MoSe2) atomic layers. MoSe2 was synthesized onto fluorine doped tin oxide substrates and could be directly used as a counter electrode (CE) for dye-sensitized solar cells (DSSCs). The role of deposition time on the growth of MoSe2 CE was elaborately discussed using Raman, X-ray diffraction and photoluminescence studies. Influence of wet chemical growth time on the surface modification of MoSe2 CE was evidently demonstrated by scanning electron microscopy and atomic force microscopy studies. The MoSe2 CE electrode has lower charge transfer resistance and superior electrocatalytic activity towards triiodide/iodide redox behavior, comparable to conventional Pt CEs. High power conversion efficiency of 7.28% was achieved, equivalent to scarce noble metal Pt CE (7.40%). Uniform surface morphology with active edge sites highly dominated to promote the superior electrocatalytic activity. This work opens a way to use an economical wet chemical method to fabricate the layered MoSe2 CE as a replacement for high cost Pt based CE for DSSCs. This paper presents a simple and large area wet chemical preparation route for molybdenum diselenide (MoSe2) atomic layers. MoSe2 was synthesized onto fluorine doped tin oxide substrates and could be directly used as a counter electrode (CE) for dye-sensitized solar cells (DSSCs). The role of deposition time on the growth of MoSe2 CE was elaborately discussed using Raman, X-ray diffraction and photoluminescence studies. Influence of wet chemical growth time on the surface modification of MoSe2 CE was evidently demonstrated by scanning electron microscopy and atomic force microscopy studies. The MoSe2 CE electrode has lower charge transfer resistance and superior electrocatalytic activity towards triiodide/iodide redox behavior, comparable to conventional Pt CEs. High power conversion efficiency of 7.28% was achieved, equivalent to scarce noble metal Pt CE (7.40%). Uniform surface morphology with active edge sites highly dominated to promote the superior electrocatalytic activity. This work opens a way to use an economical wet chemical method to fabricate the layered MoSe2 CE as a replacement for high cost Pt based CE for DSSCs. KCI Citation Count: 12 |
| Author | Jeong, Sung Hoon Park, Hui Joon Mengal, Naveed Kim, Hyun-Seok Patil, Supriya A. Jung, Jongwan Vikraman, Dhanasekaran Hussain, Sajjad Kim, Hak-Sung |
| Author_xml | – sequence: 1 givenname: Dhanasekaran orcidid: 0000-0001-8991-3604 surname: Vikraman fullname: Vikraman, Dhanasekaran organization: Division of Electronics and Electrical Engineering, Dongguk University-Seoul, Seoul 04620, Republic of Korea – sequence: 2 givenname: Supriya A. surname: Patil fullname: Patil, Supriya A. organization: Department of Mechanical Engineering, Hanyang University, Seoul 04763, Republic of Korea – sequence: 3 givenname: Sajjad surname: Hussain fullname: Hussain, Sajjad organization: Graphene Research Institute, Sejong University, Seoul 05006, Republic of Korea – sequence: 4 givenname: Naveed surname: Mengal fullname: Mengal, Naveed organization: Department of Organic and Nano Engineering, Hanyang University, Seoul 04763, Republic of Korea – sequence: 5 givenname: Sung Hoon surname: Jeong fullname: Jeong, Sung Hoon organization: Department of Organic and Nano Engineering, Hanyang University, Seoul 04763, Republic of Korea – sequence: 6 givenname: Jongwan orcidid: 0000-0002-1397-212X surname: Jung fullname: Jung, Jongwan organization: Graphene Research Institute, Sejong University, Seoul 05006, Republic of Korea – sequence: 7 givenname: Hui Joon orcidid: 0000-0003-4607-207X surname: Park fullname: Park, Hui Joon organization: Department of Energy Systems Research, Ajou University, Suwon 16499, Republic of Korea – sequence: 8 givenname: Hak-Sung surname: Kim fullname: Kim, Hak-Sung email: kima@hanyang.ac.kr organization: Department of Mechanical Engineering, Hanyang University, Seoul 04763, Republic of Korea – sequence: 9 givenname: Hyun-Seok orcidid: 0000-0003-1127-5766 surname: Kim fullname: Kim, Hyun-Seok email: hyunseokk@dongguk.edu organization: Division of Electronics and Electrical Engineering, Dongguk University-Seoul, Seoul 04620, Republic of Korea |
| BackLink | https://www.kci.go.kr/kciportal/ci/sereArticleSearch/ciSereArtiView.kci?sereArticleSearchBean.artiId=ART002435756$$DAccess content in National Research Foundation of Korea (NRF) |
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| CitedBy_id | crossref_primary_10_1016_j_mtchem_2023_101562 crossref_primary_10_1016_j_jpowsour_2025_236242 crossref_primary_10_1016_j_surfin_2022_102374 crossref_primary_10_1039_C8QI00831K crossref_primary_10_1016_j_optmat_2022_112763 crossref_primary_10_1016_j_apsusc_2019_144401 crossref_primary_10_1016_j_jmrt_2022_02_050 crossref_primary_10_1016_j_apsusc_2025_162758 crossref_primary_10_1021_acssuschemeng_9b02430 crossref_primary_10_1021_acssuschemeng_8b03921 crossref_primary_10_3390_polym12040918 crossref_primary_10_1016_j_jallcom_2020_154631 crossref_primary_10_1021_acsami_0c19890 crossref_primary_10_1002_adsu_202100025 crossref_primary_10_1016_j_apsusc_2020_148863 crossref_primary_10_1016_j_spmi_2020_106388 crossref_primary_10_1016_j_jpcs_2023_111597 crossref_primary_10_1039_D0GC01148G |
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| Keywords | Wet chemical Electrocatalytic Surface morphology MoSe2 DSSC |
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•Wet chemical methodology was used to synthesize MoSe2 as a CE for DSSCs.•High PCE of 7.28% achieves using MoSe2 CE, equivalent to Pt CE... This paper presents a simple and large area wet chemical preparation route for molybdenum diselenide (MoSe2) atomic layers. MoSe2 was synthesized onto fluorine... |
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| SubjectTerms | DSSC Electrocatalytic MoSe2 Surface morphology Wet chemical 화학공학 |
| Title | Construction of dye-sensitized solar cells using wet chemical route synthesized MoSe2 counter electrode |
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