Lifetime enhancement of exciplex based organic light-emitting diodes by triplet exciton engineering
A device approach to improve the device lifetime of exciplex organic light-emitting diodes was studied by managing the intermolecular interaction and concentration quenching of exciplexes. The exciplexes were made up of a p-type material and a bipolar n-type material, in which the ratio of the p-typ...
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| Published in | Journal of industrial and engineering chemistry (Seoul, Korea) Vol. 93; pp. 388 - 393 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
25.01.2021
한국공업화학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1226-086X 1876-794X |
| DOI | 10.1016/j.jiec.2020.10.016 |
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| Abstract | A device approach to improve the device lifetime of exciplex organic light-emitting diodes was studied by managing the intermolecular interaction and concentration quenching of exciplexes. The exciplexes were made up of a p-type material and a bipolar n-type material, in which the ratio of the p-type material was less than 50% for dispersion in the n-type material to copy the conventional host-dopant type emitting layer. The exciplexes generated between the p-type material and n-type material were dispersed in the n-type material. The device lifetime of the exciplex organic light-emitting diodes was extended by almost four times through control of the p-type material content by mimicking the host-dopant system. The analysis of the lifetime improvement mechanism revealed that suppression of triplet exciton loss by strong intermolecular interaction and concentration quenching was the major pathway to stabilize the exciplex devices by dispersion. Additionally, the device lifetime of the fluorescence emitter doped exciplex devices was extended by more than three times. Therefore, the exciplexes with a p-type material dispersed in the bipolar n-type material were effective to elongate the device lifetime of the exciplex based organic light-emitting diodes. |
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| AbstractList | A device approach to improve the device lifetime of exciplex organic light-emitting diodes was studied bymanaging the intermolecular interaction and concentration quenching of exciplexes. The exciplexes weremade up of a p-type material and a bipolar n-type material, in which the ratio of the p-type material wasless than 50% for dispersion in the n-type material to copy the conventional host-dopant type emittinglayer. The exciplexes generated between the p-type material and n-type material were dispersed in the ntypematerial. The device lifetime of the exciplex organic light-emitting diodes was extended by almostfour times through control of the p-type material content by mimicking the host-dopant system. Theanalysis of the lifetime improvement mechanism revealed that suppression of triplet exciton loss bystrong intermolecular interaction and concentration quenching was the major pathway to stabilize theexciplex devices by dispersion. Additionally, the device lifetime of thefluorescence emitter dopedexciplex devices was extended by more than three times. Therefore, the exciplexes with a p-type materialdispersed in the bipolar n-type material were effective to elongate the device lifetime of the exciplexbased organic light-emitting diodes. KCI Citation Count: 1 A device approach to improve the device lifetime of exciplex organic light-emitting diodes was studied by managing the intermolecular interaction and concentration quenching of exciplexes. The exciplexes were made up of a p-type material and a bipolar n-type material, in which the ratio of the p-type material was less than 50% for dispersion in the n-type material to copy the conventional host-dopant type emitting layer. The exciplexes generated between the p-type material and n-type material were dispersed in the n-type material. The device lifetime of the exciplex organic light-emitting diodes was extended by almost four times through control of the p-type material content by mimicking the host-dopant system. The analysis of the lifetime improvement mechanism revealed that suppression of triplet exciton loss by strong intermolecular interaction and concentration quenching was the major pathway to stabilize the exciplex devices by dispersion. Additionally, the device lifetime of the fluorescence emitter doped exciplex devices was extended by more than three times. Therefore, the exciplexes with a p-type material dispersed in the bipolar n-type material were effective to elongate the device lifetime of the exciplex based organic light-emitting diodes. |
| Author | Jang, Ho Jin Lee, Jun Yeob |
| Author_xml | – sequence: 1 givenname: Ho Jin surname: Jang fullname: Jang, Ho Jin – sequence: 2 givenname: Jun Yeob surname: Lee fullname: Lee, Jun Yeob email: leej17@skku.edu |
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| Cites_doi | 10.1080/15980316.2019.1680453 10.1002/adom.201500634 10.1063/1.2786840 10.1021/acs.jpcc.9b08261 10.1016/j.jiec.2020.02.021 10.1080/15980316.2019.1572662 10.1038/nphoton.2012.31 10.1021/acsami.7b16887 10.1021/acsami.7b18318 10.1002/adma.201300753 10.1002/adfm.201505014 10.1007/s13233-019-7045-0 10.1021/acs.jpcc.7b02369 10.1039/C7TC00556C 10.1039/C6CS00368K 10.1016/j.orgel.2016.09.020 10.1063/1.1467614 10.1002/adma.201803524 10.1039/C9TC03808F 10.1126/sciadv.1501470 10.1016/j.orgel.2019.105477 10.3390/app8091449 10.1016/j.orgel.2017.06.057 10.1038/nature11687 10.1021/acs.jpcc.0c04196 10.1016/j.orgel.2017.09.013 |
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