Mid-infrared CO2 sensor with blended absorption features for non-uniform laminar premixed flames
We develop a novel mid-infrared CO 2 absorption sensor exploiting spectrally blended features to characterize thermochemical non-uniformity of laminar premixed flames. A new algorithm for interpreting spectra with significantly blended features is proposed for single line-of-sight multi-transition a...
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| Published in | Applied physics. B, Lasers and optics Vol. 128; no. 2 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Berlin/Heidelberg
Springer Berlin Heidelberg
01.02.2022
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0946-2171 1432-0649 |
| DOI | 10.1007/s00340-022-07758-2 |
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| Abstract | We develop a novel mid-infrared CO
2
absorption sensor exploiting spectrally blended features to characterize thermochemical non-uniformity of laminar premixed flames. A new algorithm for interpreting spectra with significantly blended features is proposed for single line-of-sight multi-transition absorption thermometry. A CO
2
sensor covering eight absorption transitions near 2378.0 cm
−1
is demonstrated in a laminar premixed CH
4
/Air flame at an equivalence ratio of
φ
=
1.0
. The average signal-to-noise ratio is 1293 with a measurement time of 1.0 s, and the estimated CO
2
detection limit is 42.8 ppm at 1543 K with 6 cm pathlength. Computational fluid dynamics (CFD) simulation with reduced GRI 1.2 mechanism is performed for comparison. Spatially resolved distributions are obtained with the laser absorption spectroscopy (LAS) measurements, combined with postulated distribution from CFD simulation. The LAS measurements agree with the CFD simulation, with a central-zone temperature difference of less than 1.1% and CO
2
concentration difference of less than 1.0%. Discrepancy is observed in the boundary layer region due to pronounced mixing with the ambient surroundings. The sensor developed provides a lead for general LAS sensor design (blended absorption features, ambient interference, or under optically thick conditions), and can serve for practical combustion sensing. |
|---|---|
| AbstractList | We develop a novel mid-infrared CO2 absorption sensor exploiting spectrally blended features to characterize thermochemical non-uniformity of laminar premixed flames. A new algorithm for interpreting spectra with significantly blended features is proposed for single line-of-sight multi-transition absorption thermometry. A CO2 sensor covering eight absorption transitions near 2378.0 cm−1 is demonstrated in a laminar premixed CH4/Air flame at an equivalence ratio of φ=1.0. The average signal-to-noise ratio is 1293 with a measurement time of 1.0 s, and the estimated CO2 detection limit is 42.8 ppm at 1543 K with 6 cm pathlength. Computational fluid dynamics (CFD) simulation with reduced GRI 1.2 mechanism is performed for comparison. Spatially resolved distributions are obtained with the laser absorption spectroscopy (LAS) measurements, combined with postulated distribution from CFD simulation. The LAS measurements agree with the CFD simulation, with a central-zone temperature difference of less than 1.1% and CO2 concentration difference of less than 1.0%. Discrepancy is observed in the boundary layer region due to pronounced mixing with the ambient surroundings. The sensor developed provides a lead for general LAS sensor design (blended absorption features, ambient interference, or under optically thick conditions), and can serve for practical combustion sensing. We develop a novel mid-infrared CO 2 absorption sensor exploiting spectrally blended features to characterize thermochemical non-uniformity of laminar premixed flames. A new algorithm for interpreting spectra with significantly blended features is proposed for single line-of-sight multi-transition absorption thermometry. A CO 2 sensor covering eight absorption transitions near 2378.0 cm −1 is demonstrated in a laminar premixed CH 4 /Air flame at an equivalence ratio of φ = 1.0 . The average signal-to-noise ratio is 1293 with a measurement time of 1.0 s, and the estimated CO 2 detection limit is 42.8 ppm at 1543 K with 6 cm pathlength. Computational fluid dynamics (CFD) simulation with reduced GRI 1.2 mechanism is performed for comparison. Spatially resolved distributions are obtained with the laser absorption spectroscopy (LAS) measurements, combined with postulated distribution from CFD simulation. The LAS measurements agree with the CFD simulation, with a central-zone temperature difference of less than 1.1% and CO 2 concentration difference of less than 1.0%. Discrepancy is observed in the boundary layer region due to pronounced mixing with the ambient surroundings. The sensor developed provides a lead for general LAS sensor design (blended absorption features, ambient interference, or under optically thick conditions), and can serve for practical combustion sensing. |
| ArticleNumber | 31 |
| Author | Wang, Weitian Ma, Liuhao Ren, Wei Chao, Xing Fu, Pengfei Wang, Zhenhai |
| Author_xml | – sequence: 1 givenname: Zhenhai surname: Wang fullname: Wang, Zhenhai organization: Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Energy and Power Engineering, Center for Combustion Energy, Tsinghua University – sequence: 2 givenname: Weitian surname: Wang fullname: Wang, Weitian organization: Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Energy and Power Engineering, Center for Combustion Energy, Tsinghua University – sequence: 3 givenname: Liuhao surname: Ma fullname: Ma, Liuhao organization: School of Automotive Engineering, Wuhan University of Technology – sequence: 4 givenname: Pengfei surname: Fu fullname: Fu, Pengfei organization: School of Aerospace Engineering, Tsinghua University – sequence: 5 givenname: Wei surname: Ren fullname: Ren, Wei organization: Department of Mechanical and Automation Engineering, Shenzhen Research Institute, The Chinese University of Hong Kong – sequence: 6 givenname: Xing orcidid: 0000-0003-1120-8803 surname: Chao fullname: Chao, Xing email: chaox6@tsinghua.edu.cn organization: Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Energy and Power Engineering, Center for Combustion Energy, Tsinghua University |
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| Snippet | We develop a novel mid-infrared CO
2
absorption sensor exploiting spectrally blended features to characterize thermochemical non-uniformity of laminar premixed... We develop a novel mid-infrared CO2 absorption sensor exploiting spectrally blended features to characterize thermochemical non-uniformity of laminar premixed... |
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| SubjectTerms | Algorithms Applied physics Boundary layers Carbon dioxide Carbon dioxide concentration Computational fluid dynamics Engineering Equivalence ratio Infrared detectors Lasers Nonuniformity Optical Devices Optics Photonics Physical Chemistry Physics Physics and Astronomy Premixed flames Quantum Optics Sensors Signal to noise ratio Simulation Spectrum analysis |
| Title | Mid-infrared CO2 sensor with blended absorption features for non-uniform laminar premixed flames |
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