Rotational motion of polyanion versus volume effect associated with ionic conductivity of several solid electrolytes
Volume effect has been extensively investigated in several families of solid electrolytes, i.e., expanding the skeleton lattice by bigger-size substitution favors the ionic conduction. However, this effect is not applicable in α-Li 2 SO 4 and α-Na 3 PO 4 based inorganic ionic plastic crystal electro...
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| Published in | Rare metals Vol. 37; no. 6; pp. 497 - 503 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
Nonferrous Metals Society of China
01.06.2018
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1001-0521 1867-7185 |
| DOI | 10.1007/s12598-018-1058-2 |
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| Abstract | Volume effect has been extensively investigated in several families of solid electrolytes, i.e., expanding the skeleton lattice by bigger-size substitution favors the ionic conduction. However, this effect is not applicable in α-Li
2
SO
4
and α-Na
3
PO
4
based inorganic ionic plastic crystal electrolytes, a unique family of solid electrolytes. Here, it is proposed that the underlying rotational motion effect of polyanion, which is actually inhibited by the substitution of bigger-size polyanion in single-phase solid solution region and causes the unexpected lowering of the ionic conductivity instead, should need the more consideration. Furthermore, through utilizing the rotational motion effect of polyanion, it is given that a new explanation of the ionic conductivities of Li
10
MP
2
S
12
(M = Si, Ge, Se) electrolytes deviating from the volume effect. These results inspire new vision of rationalization of the high-performance solid electrolytes by tuning the rotational motion effect of polyanion. |
|---|---|
| AbstractList | Volume effect has been extensively investigated in several families of solid electrolytes, i.e., expanding the skeleton lattice by bigger-size substitution favors the ionic conduction. However, this effect is not applicable in α-Li
2
SO
4
and α-Na
3
PO
4
based inorganic ionic plastic crystal electrolytes, a unique family of solid electrolytes. Here, it is proposed that the underlying rotational motion effect of polyanion, which is actually inhibited by the substitution of bigger-size polyanion in single-phase solid solution region and causes the unexpected lowering of the ionic conductivity instead, should need the more consideration. Furthermore, through utilizing the rotational motion effect of polyanion, it is given that a new explanation of the ionic conductivities of Li
10
MP
2
S
12
(M = Si, Ge, Se) electrolytes deviating from the volume effect. These results inspire new vision of rationalization of the high-performance solid electrolytes by tuning the rotational motion effect of polyanion. Volume effect has been extensively investigated in several families of solid electrolytes, i.e., expanding the skeleton lattice by bigger-size substitution favors the ionic conduction. However, this effect is not applicable in α-Li2SO4 and α-Na3PO4 based inorganic ionic plastic crystal electrolytes, a unique family of solid electrolytes. Here, it is proposed that the underlying rotational motion effect of polyanion, which is actually inhibited by the substitution of bigger-size polyanion in single-phase solid solution region and causes the unexpected lowering of the ionic conductivity instead, should need the more consideration. Furthermore, through utilizing the rotational motion effect of polyanion, it is given that a new explanation of the ionic conductivities of Li10MP2S12 (M = Si, Ge, Se) electrolytes deviating from the volume effect. These results inspire new vision of rationalization of the high-performance solid electrolytes by tuning the rotational motion effect of polyanion. |
| Author | Shi, Si-Qi Chen, Li-Quan Li, Yuan-Ji Pan, Li Zhao, Qian |
| Author_xml | – sequence: 1 givenname: Qian surname: Zhao fullname: Zhao, Qian organization: Materials Genome Institute, Shanghai University – sequence: 2 givenname: Li surname: Pan fullname: Pan, Li organization: School of Materials Science and Engineering, Shanghai University – sequence: 3 givenname: Yuan-Ji surname: Li fullname: Li, Yuan-Ji organization: Qianweichang College, Shanghai University – sequence: 4 givenname: Li-Quan surname: Chen fullname: Chen, Li-Quan organization: Institute of Physics, Chinese Academy of Sciences – sequence: 5 givenname: Si-Qi orcidid: 0000-0001-8988-9763 surname: Shi fullname: Shi, Si-Qi email: sqshi@shu.edu.cn organization: Materials Genome Institute, Shanghai University, School of Materials Science and Engineering, Shanghai University |
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| Keywords | Volume effect Inorganic plastic crystal electrolyte Rotational motion of polyanion Ionic conductivity |
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| SubjectTerms | Biomaterials Chemistry and Materials Science Electrolytes Energy Germanium Ion currents Ions Materials Engineering Materials Science Metallic Materials Molten salt electrolytes Nanoscale Science and Technology Physical Chemistry Silicon Sodium phosphate Solid electrolytes Solid solutions Substitutes |
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