Stress effects on the kinetics of hydrogen adsorption in a spherical particle: An analytical model

We consider a two-phase elastic solid subject to diffusion-induced phase transformation by interstitial hydrogen. We derive a simple analytical model to quantify the effect of misfit strain on the kinetic of phase transformation and to calculate the amplitude of the well-know hysteresis cycle observ...

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Published inInternational journal of hydrogen energy Vol. 40; no. 47; pp. 17009 - 17016
Main Authors Duda, Fernando P., Tomassetti, Giuseppe
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 21.12.2015
Subjects
Online AccessGet full text
ISSN0360-3199
1879-3487
DOI10.1016/j.ijhydene.2015.07.088

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Abstract We consider a two-phase elastic solid subject to diffusion-induced phase transformation by interstitial hydrogen. We derive a simple analytical model to quantify the effect of misfit strain on the kinetic of phase transformation and to calculate the amplitude of the well-know hysteresis cycle observed when a sequence of forward and reverse phase transformations takes place. •We consider adsorption and desorption of interstitial hydrogen by a spherical particle.•The particle is modeled as a two-phase elastic solid partitioned by a sharp interface.•Elastic misfits are taken into account.•A differential equation governing the motion of the phase interface is derived.•A closed-form solution is obtained.
AbstractList We consider a two-phase elastic solid subject to diffusion-induced phase transformation by interstitial hydrogen. We derive a simple analytical model to quantify the effect of misfit strain on the kinetic of phase transformation and to calculate the amplitude of the well-know hysteresis cycle observed when a sequence of forward and reverse phase transformations takes place. •We consider adsorption and desorption of interstitial hydrogen by a spherical particle.•The particle is modeled as a two-phase elastic solid partitioned by a sharp interface.•Elastic misfits are taken into account.•A differential equation governing the motion of the phase interface is derived.•A closed-form solution is obtained.
Author Tomassetti, Giuseppe
Duda, Fernando P.
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  organization: Università di Roma “Tor Vergata”, Dipartimento di Ingegneria Civile e Ingegneria Informatica, Via Politecnico 1, 00169, Italy
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Issue 47
Keywords Nanoparticles
Phase transformation
Hydrogen storage
Stress-assisted diffusion
Hysteresis
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Snippet We consider a two-phase elastic solid subject to diffusion-induced phase transformation by interstitial hydrogen. We derive a simple analytical model to...
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SubjectTerms Hydrogen storage
Hysteresis
Nanoparticles
Phase transformation
Stress-assisted diffusion
Title Stress effects on the kinetics of hydrogen adsorption in a spherical particle: An analytical model
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