Influence of eco-friendly agar-derivatives on the electrochemical performance of carbon felts electrodes of vanadium redox flow battery
In this study, bio-derived natural agar powder was used as an electrocatalyst for application as an electrode in all‑vanadium redox flow batteries. Different concentrations of agar solution were tested, and cyclic voltammetry studies confirmed that agar loaded felts have good catalytic activity towa...
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| Published in | Journal of energy storage Vol. 84; p. 110599 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
15.04.2024
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| Subjects | |
| Online Access | Get full text |
| ISSN | 2352-152X 2352-1538 |
| DOI | 10.1016/j.est.2024.110599 |
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| Abstract | In this study, bio-derived natural agar powder was used as an electrocatalyst for application as an electrode in all‑vanadium redox flow batteries. Different concentrations of agar solution were tested, and cyclic voltammetry studies confirmed that agar loaded felts have good catalytic activity toward both redox couples V4+/V5+ at the positive and V2+/V3+ at the negative side. Energy dispersive X-ray spectroscopy and X-ray photoelectron spectroscopy demonstrated the presence of higher amount of oxygen-functional groups on the surface of the fibers. Contact angle measurements demonstrated an enormous increase in hydrophilicity of the felts treated with agar. Long-term charge/discharge profiles revealed 6 % higher energy efficiency and 13 % better discharge capacity retention for agar modified felts when compared to thermally treated carbon felts at a relatively high current density of 150 mA cm−2.
•Enormous increase in hydrophilicity of carbon felt is achieved.•High energy efficiency and discharge capacity are reported at high current density.•Stable enhancement in VRFB performance is evident.•Lower charge transfer resistance is reported. |
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| AbstractList | In this study, bio-derived natural agar powder was used as an electrocatalyst for application as an electrode in all‑vanadium redox flow batteries. Different concentrations of agar solution were tested, and cyclic voltammetry studies confirmed that agar loaded felts have good catalytic activity toward both redox couples V4+/V5+ at the positive and V2+/V3+ at the negative side. Energy dispersive X-ray spectroscopy and X-ray photoelectron spectroscopy demonstrated the presence of higher amount of oxygen-functional groups on the surface of the fibers. Contact angle measurements demonstrated an enormous increase in hydrophilicity of the felts treated with agar. Long-term charge/discharge profiles revealed 6 % higher energy efficiency and 13 % better discharge capacity retention for agar modified felts when compared to thermally treated carbon felts at a relatively high current density of 150 mA cm−2.
•Enormous increase in hydrophilicity of carbon felt is achieved.•High energy efficiency and discharge capacity are reported at high current density.•Stable enhancement in VRFB performance is evident.•Lower charge transfer resistance is reported. |
| ArticleNumber | 110599 |
| Author | Matouk, Zineb Bahaa, Ahmed Alhammadi, Ayoob Andisetiawan, Anugrah Fetyan, Abdulmonem |
| Author_xml | – sequence: 1 givenname: Abdulmonem surname: Fetyan fullname: Fetyan, Abdulmonem email: Abdulmonem.fetyan@dewa.gov.ae, Abdulmonem.fetyan@zu.ac.ae organization: Research & Development Centre, Dubai Electricity and Water Authority (DEWA), P.O. Box 564, Dubai, United Arab Emirates – sequence: 2 givenname: Ayoob surname: Alhammadi fullname: Alhammadi, Ayoob organization: Research & Development Centre, Dubai Electricity and Water Authority (DEWA), P.O. Box 564, Dubai, United Arab Emirates – sequence: 3 givenname: Zineb surname: Matouk fullname: Matouk, Zineb organization: Technology innovation institute, P.O. Box: 9639, Masdar City, Abu Dhabi, United Arab Emirates – sequence: 4 givenname: Anugrah surname: Andisetiawan fullname: Andisetiawan, Anugrah organization: Research & Development Centre, Dubai Electricity and Water Authority (DEWA), P.O. Box 564, Dubai, United Arab Emirates – sequence: 5 givenname: Ahmed surname: Bahaa fullname: Bahaa, Ahmed organization: Research & Development Centre, Dubai Electricity and Water Authority (DEWA), P.O. Box 564, Dubai, United Arab Emirates |
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| CitedBy_id | crossref_primary_10_1002_cssc_202401010 crossref_primary_10_1002_ente_202401465 crossref_primary_10_3390_su162411289 |
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| Keywords | Agar Redox flow batteries Electrode Bio-derived polymer Carbon felt |
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| Snippet | In this study, bio-derived natural agar powder was used as an electrocatalyst for application as an electrode in all‑vanadium redox flow batteries. Different... |
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| SubjectTerms | Agar Bio-derived polymer Carbon felt Electrode Redox flow batteries |
| Title | Influence of eco-friendly agar-derivatives on the electrochemical performance of carbon felts electrodes of vanadium redox flow battery |
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