Tb(III) functionalized MOF based self-calibrating sensor integrated with logic gate operation for efficient epinephrine detection in serum
By anchoring Tb3+ ions on its free carboxyl groups of the nanocaged NiMOF, a dual-emission self-calibrating sensor of Tb3+@NiMOF was fabricated through coordination post-synthetic modification (PSM) strategy. With Tb3+ ions as the secondary fluorescent signal and sensing active sites, Tb3+@NiMOF pre...
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| Published in | Journal of rare earths Vol. 42; no. 5; pp. 987 - 994 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.05.2024
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1002-0721 2509-4963 |
| DOI | 10.1016/j.jre.2023.04.007 |
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| Abstract | By anchoring Tb3+ ions on its free carboxyl groups of the nanocaged NiMOF, a dual-emission self-calibrating sensor of Tb3+@NiMOF was fabricated through coordination post-synthetic modification (PSM) strategy. With Tb3+ ions as the secondary fluorescent signal and sensing active sites, Tb3+@NiMOF presents great potentials in visually and efficiently monitoring EPI in serum, with high sensitivity and selectivity, fast response, excellent recyclable, and the low detection limit (LOD, 3.06 ng/mL). Furthermore, a tandem combinational logic gate based intelligent detection system was constructed to improve the practicability and convenience of epinephrine (EPI) detection in serum by comparing the light emitted colour with the series standard colour cards preset in the smartphone. This work provides a promising approach of developing metal–organic frameworks (MOFs) based self-calibrating sensors for intelligent detection of bioactive molecules.
A dual-emission self-calibrating sensor of Tb3+@NiMOF integrated with the tandem combinational logic gate operation to detect epinephrine in serum efficiently with high reliability, high sensitivity, and low detection limits. [Display omitted] |
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| AbstractList | By anchoring Tb3+ ions on its free carboxyl groups of the nanocaged NiMOF, a dual-emission self-calibrating sensor of Tb3+@NiMOF was fabricated through coordination post-synthetic modification (PSM) strategy. With Tb3+ ions as the secondary fluorescent signal and sensing active sites, Tb3+@NiMOF presents great potentials in visually and efficiently monitoring EPI in serum, with high sensitivity and selectivity, fast response, excellent recyclable, and the low detection limit (LOD, 3.06 ng/mL). Furthermore, a tandem combinational logic gate based intelligent detection system was constructed to improve the practicability and convenience of epinephrine (EPI) detection in serum by comparing the light emitted colour with the series standard colour cards preset in the smartphone. This work provides a promising approach of developing metal–organic frameworks (MOFs) based self-calibrating sensors for intelligent detection of bioactive molecules.
A dual-emission self-calibrating sensor of Tb3+@NiMOF integrated with the tandem combinational logic gate operation to detect epinephrine in serum efficiently with high reliability, high sensitivity, and low detection limits. [Display omitted] |
| Author | Li, Wenqian Fan, Liming Zhao, Dongsheng Li, Wencui Liu, Xin Wen, Rongmei Zhang, Xiutang |
| Author_xml | – sequence: 1 givenname: Dongsheng surname: Zhao fullname: Zhao, Dongsheng organization: Shanxi Key Laboratory of Advanced Carbon Electrode Materials, Shanxi Coal Mine Water Treatment Technology Innovation Center, School of Chemistry and Chemical Engineering, North University of China, Taiyuan, 030051, China – sequence: 2 givenname: Wenqian surname: Li fullname: Li, Wenqian organization: Shanxi Key Laboratory of Advanced Carbon Electrode Materials, Shanxi Coal Mine Water Treatment Technology Innovation Center, School of Chemistry and Chemical Engineering, North University of China, Taiyuan, 030051, China – sequence: 3 givenname: Rongmei surname: Wen fullname: Wen, Rongmei organization: Shanxi Key Laboratory of Advanced Carbon Electrode Materials, Shanxi Coal Mine Water Treatment Technology Innovation Center, School of Chemistry and Chemical Engineering, North University of China, Taiyuan, 030051, China – sequence: 4 givenname: Wencui surname: Li fullname: Li, Wencui organization: Shanxi Key Laboratory of Advanced Carbon Electrode Materials, Shanxi Coal Mine Water Treatment Technology Innovation Center, School of Chemistry and Chemical Engineering, North University of China, Taiyuan, 030051, China – sequence: 5 givenname: Xin surname: Liu fullname: Liu, Xin organization: Shanxi Key Laboratory of Advanced Carbon Electrode Materials, Shanxi Coal Mine Water Treatment Technology Innovation Center, School of Chemistry and Chemical Engineering, North University of China, Taiyuan, 030051, China – sequence: 6 givenname: Xiutang surname: Zhang fullname: Zhang, Xiutang email: xiutangzhang@163.com organization: Shanxi Key Laboratory of Advanced Carbon Electrode Materials, Shanxi Coal Mine Water Treatment Technology Innovation Center, School of Chemistry and Chemical Engineering, North University of China, Taiyuan, 030051, China – sequence: 7 givenname: Liming orcidid: 0000-0003-4615-0533 surname: Fan fullname: Fan, Liming email: limingfan@nuc.edu.cn organization: Shanxi Key Laboratory of Advanced Carbon Electrode Materials, Shanxi Coal Mine Water Treatment Technology Innovation Center, School of Chemistry and Chemical Engineering, North University of China, Taiyuan, 030051, China |
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| Copyright | 2023 Chinese Society of Rare Earths |
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| Keywords | Logic gate operation Epinephrine detection Self-calibrating sensor Metal-organic framework Rare earths Post-synthetic modification |
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| SubjectTerms | Epinephrine detection Logic gate operation Metal-organic framework Post-synthetic modification Rare earths Self-calibrating sensor |
| Title | Tb(III) functionalized MOF based self-calibrating sensor integrated with logic gate operation for efficient epinephrine detection in serum |
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