Modeling of methane steam reforming in a microchannel subject to multicomponent diffusion
Catalytic methane steam reforming in a slot microchannel under external heat supply to the mixture reacting on walls is considered based on numerical simulation of a complete system of Navier-Stokes equations. Three ways of heat supply to channel walls are represented, namely, a uniform heat flux, a...
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| Published in | Journal of engineering thermophysics Vol. 20; no. 3; pp. 229 - 239 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Dordrecht
SP MAIK Nauka/Interperiodica
01.09.2011
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1810-2328 1990-5432 |
| DOI | 10.1134/S1810232811030015 |
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| Abstract | Catalytic methane steam reforming in a slot microchannel under external heat supply to the mixture reacting on walls is considered based on numerical simulation of a complete system of Navier-Stokes equations. Three ways of heat supply to channel walls are represented, namely, a uniform heat flux, a heat flux linearly decreasing in channel length, and a heat flux following the reaction rate profile of the main reaction. The thermophysical parameters of the mixture depend on its temperature and composition. Two diffusion models are considered, namely, models with equal and different diffusion coefficients for each mixture component. It is shown that consideration of multicomponent diffusion does not practically affect the concentration of the components and the methane reforming at the outlet. For the above-mentioned ways of heat supply, the methane reforming with a heat flux linearly decreasing in channel length is most significant. |
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| AbstractList | Catalytic methane steam reforming in a slot microchannel under external heat supply to the mixture reacting on walls is considered based on numerical simulation of a complete system of Navier-Stokes equations. Three ways of heat supply to channel walls are represented, namely, a uniform heat flux, a heat flux linearly decreasing in channel length, and a heat flux following the reaction rate profile of the main reaction. The thermophysical parameters of the mixture depend on its temperature and composition. Two diffusion models are considered, namely, models with equal and different diffusion coefficients for each mixture component. It is shown that consideration of multicomponent diffusion does not practically affect the concentration of the components and the methane reforming at the outlet. For the above-mentioned ways of heat supply, the methane reforming with a heat flux linearly decreasing in channel length is most significant. |
| Author | Kuznetsov, V. V. Kozlov, S. P. |
| Author_xml | – sequence: 1 givenname: V. V. surname: Kuznetsov fullname: Kuznetsov, V. V. email: vladkuz@itp.nsc.ru organization: Kutateladze Institute of Thermophysics, Siberian Branch, Russian Academy of Sciences – sequence: 2 givenname: S. P. surname: Kozlov fullname: Kozlov, S. P. organization: Kutateladze Institute of Thermophysics, Siberian Branch, Russian Academy of Sciences |
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| Cites_doi | 10.1016/S1385-8947(00)00367-3 10.1021/ie50677a007 10.1002/aic.690441114 10.1063/1.1747673 10.1002/aic.690390708 10.1134/S1810232807020075 10.1109/JMEMS.2006.878888 10.1002/aic.690350109 10.1016/j.jpowsour.2004.10.018 10.1063/1.1724352 |
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| Keywords | Channel Length Mixture Temperature Engineer THERMOPHYSICS Thermophysical Parameter Heat Supply |
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| References_xml | – reference: HouK.H.HughesR.The Kinetics of Methane Steam Reforming over a Ni/_-Al2O3 CatalystChem. Eng. J.20018231132810.1016/S1385-8947(00)00367-3 – reference: MasonE.A.SaxenaS.C.Formula for the Thermal Conductivity of Gas MixturesThe Phys. Fluids195813613691114691958PhFl....1..361M10.1063/1.1724352 – reference: XuJ.FromentG.F.Methane Steam Reforming, Methanation and Water-Gas Shift, I. Intrinsic KineticsAiche J.1989351889610.1002/aic.690350109 – reference: HickmanD.A.SchmidtL.D.Steps in Ch4 Oxidation on Pt and Rh Surfaces—High-Temperature Reactor SimulationsAiche J.19933971164117710.1002/aic.690390708 – reference: ArutyunovV.S.KrylovO.V.Okislitelnye prevrashcheniya metana1998MoscowNauka(Oxidation Methane Conversions) – reference: Igumnov, V.S. and Vizel’, Ya.M., Catalytic Hydrocarbon Conversion in a Heated Tube with Vapor-Gas Ratio Close to Stoichiometric, Kat. Prom., 2010, no. 6, pp. 34–40. – reference: Alaa-Eldin, M.A., Grace, J.R., Lim, C.J., and Elnashaie, S.S., Fluidized Bed Reaction System for Steam/Hydrocarbon Gas Reforming to Produce Hydrogen, US Patent 5,326,550, 1994. – reference: FullerE.N.SchettlerP.D.GiddingsJ.C.A New Method for the Prediction of Gas Phase Diffusion CoefficientsInd. Eng. Chem.1966585192710.1021/ie50677a007 – reference: WilkeC.R.Viscosity Equation for Gas MixturesJ. Chem. Phys.1950185175191950JChPh..18..517W10.1063/1.1747673 – reference: KuznetsovV.V.VitovskyO.V.DimovS.V.SafonovS.A.KozlovS.P.Hydrodynamics and Heat and Mass Transfer at Chemical Conversions in Slot ReactorsJ. Eng. Therm.20071629910610.1134/S1810232807020075 – reference: ChaniotisA.D.PoulikakosD.Catalytic Partial Oxidation Methane Reforming for Fuel CellsJ. Power Sources200514218419310.1016/j.jpowsour.2004.10.018 – reference: VagrafticN.B.A Reference Book on Thermophysical Properties of Gases and Liquids1972MoscowNauka – reference: DeutschmannO.SchmidtL.D.Modeling the Partial Oxidation of Methane in a Short-Contact-Time ReactorAiche J.199844112465247710.1002/aic.690441114 – reference: KuznetsovV.V.KozlovS.P.Modeling of Methane Steam Reforming in a Microchannel with a Heat Flow Distributed in LengthJ. Eng. Therm.200817153592435210 – reference: ReidR.C.SherwoodT.K.The Properties of Gases and Liquids1966New YorkMcGraw-Hill – reference: HyungG.P.MalenJ.A.PiggottW.T.Methanol Steam Reformer on a Silicon WaferJ. Microelectromech. Syst.200615497698510.1109/JMEMS.2006.878888 – volume-title: A Reference Book on Thermophysical Properties of Gases and Liquids year: 1972 ident: 4094_CR12 – volume: 82 start-page: 311 year: 2001 ident: 4094_CR16 publication-title: Chem. Eng. J. doi: 10.1016/S1385-8947(00)00367-3 – volume: 58 start-page: 19 issue: 5 year: 1966 ident: 4094_CR13 publication-title: Ind. Eng. Chem. doi: 10.1021/ie50677a007 – volume: 44 start-page: 2465 issue: 11 year: 1998 ident: 4094_CR7 publication-title: Aiche J. doi: 10.1002/aic.690441114 – volume: 17 start-page: 53 issue: 1 year: 2008 ident: 4094_CR5 publication-title: J. Eng. Therm. – ident: 4094_CR4 – ident: 4094_CR2 – volume: 18 start-page: 517 year: 1950 ident: 4094_CR10 publication-title: J. Chem. Phys. doi: 10.1063/1.1747673 – volume: 39 start-page: 1164 issue: 7 year: 1993 ident: 4094_CR6 publication-title: Aiche J. doi: 10.1002/aic.690390708 – volume: 16 start-page: 99 issue: 2 year: 2007 ident: 4094_CR3 publication-title: J. Eng. Therm. doi: 10.1134/S1810232807020075 – volume: 15 start-page: 976 issue: 4 year: 2006 ident: 4094_CR9 publication-title: J. Microelectromech. Syst. doi: 10.1109/JMEMS.2006.878888 – volume-title: Okislitelnye prevrashcheniya metana year: 1998 ident: 4094_CR1 – volume: 35 start-page: 88 issue: 1 year: 1989 ident: 4094_CR15 publication-title: Aiche J. doi: 10.1002/aic.690350109 – volume: 142 start-page: 184 year: 2005 ident: 4094_CR8 publication-title: J. Power Sources doi: 10.1016/j.jpowsour.2004.10.018 – volume: 1 start-page: 361 year: 1958 ident: 4094_CR11 publication-title: The Phys. Fluids doi: 10.1063/1.1724352 – volume-title: The Properties of Gases and Liquids year: 1966 ident: 4094_CR14 |
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| Title | Modeling of methane steam reforming in a microchannel subject to multicomponent diffusion |
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