MWCNT Doped Reverse-Mode Polymer Network Liquid Crystals with Frequency Response Property
Polymer-liquid crystals (PLCs) are common materials for smart windows. However, PLC smart windows usually require high driving voltage to maintain transparency. We synthesized a novel PLC smart film by doping multi-wall carbon nanotubes (MWCNTs) into a reverse-mode polymer network liquid crystal (R-...
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| Published in | Chinese physics letters Vol. 41; no. 3; pp. 38501 - 170 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Chinese Physical Society and IOP Publishing Ltd
01.03.2024
|
| Online Access | Get full text |
| ISSN | 0256-307X 1741-3540 |
| DOI | 10.1088/0256-307X/41/3/038501 |
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| Abstract | Polymer-liquid crystals (PLCs) are common materials for smart windows. However, PLC smart windows usually require high driving voltage to maintain transparency. We synthesized a novel PLC smart film by doping multi-wall carbon nanotubes (MWCNTs) into a reverse-mode polymer network liquid crystal (R-PNLC). It is found that doping MWCNTs could effectively reduce the threshold voltage (
V
th
) of R-PNLC from 19.0 V to 8.4 V. Due to co-orientation between MWCNT and LC molecules, the doped R-PNLC is able to maintain a high transmittance of visible light (∼ 80%) without an applied electric field. We find that doping MWCNTs could change the frequency modulation property of R-PNLC. The doped R-PNLC exhibits a wider frequency modulation range up to 40000 Hz, while the frequency modulation of the undoped R-PNLC reached to a saturation at 23000 Hz. We also tested the electromagnetic interference (EMI) shielding efficiency of R-PNLC and find that the EMI shielding efficiency could be improved by doping only 0.01 wt% MWCNTs into the system. The total shielding effectiveness of 0.01 wt% MWCNT doped R-PNLC was up to 14.91 dB in the frequency band of 5.38–8.17 GHz. This study demonstrates that the films are potentially useful for low-energy-consumption smart windows with enhanced electromagnetic shielding capability. |
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| AbstractList | Polymer-liquid crystals (PLCs) are common materials for smart windows. However, PLC smart windows usually require high driving voltage to maintain transparency. We synthesized a novel PLC smart film by doping multi-wall carbon nanotubes (MWCNTs) into a reverse-mode polymer network liquid crystal (R-PNLC). It is found that doping MWCNTs could effectively reduce the threshold voltage (
V
th
) of R-PNLC from 19.0 V to 8.4 V. Due to co-orientation between MWCNT and LC molecules, the doped R-PNLC is able to maintain a high transmittance of visible light (∼ 80%) without an applied electric field. We find that doping MWCNTs could change the frequency modulation property of R-PNLC. The doped R-PNLC exhibits a wider frequency modulation range up to 40000 Hz, while the frequency modulation of the undoped R-PNLC reached to a saturation at 23000 Hz. We also tested the electromagnetic interference (EMI) shielding efficiency of R-PNLC and find that the EMI shielding efficiency could be improved by doping only 0.01 wt% MWCNTs into the system. The total shielding effectiveness of 0.01 wt% MWCNT doped R-PNLC was up to 14.91 dB in the frequency band of 5.38–8.17 GHz. This study demonstrates that the films are potentially useful for low-energy-consumption smart windows with enhanced electromagnetic shielding capability. Polymer-liquid crystals(PLCs)are common materials for smart windows.However,PLC smart windows usually require high driving voltage to maintain transparency.We synthesized a novel PLC smart film by doping multi-wall carbon nanotubes(MWCNTs)into a reverse-mode polymer network liquid crystal(R-PNLC).It is found that doping MWCNTs could effectively reduce the threshold voltage(Vth)of R-PNLC from 19.0 V to 8.4 V.Due to co-orientation between MWCNT and LC molecules,the doped R-PNLC is able to maintain a high transmittance of visible light(～80％)without an applied electric field.We find that doping MWCNTs could change the frequency modulation property of R-PNLC.The doped R-PNLC exhibits a wider frequency modulation range up to 40000 Hz,while the frequency modulation of the undoped R-PNLC reached to a saturation at 23000 Hz.We also tested the electromagnetic interference(EMI)shielding efficiency of R-PNLC and find that the EMI shielding efficiency could be improved by doping only 0.01 wt％MWCNTs into the system.The total shielding effectiveness of 0.01 wt％MWCNT doped R-PNLC was up to 14.91 dB in the frequency band of 5.38-8.17 GHz.This study demonstrates that the films are potentially useful for low-energy-consumption smart windows with enhanced electromagnetic shielding capability. |
| Author | Wang, Tianyu Zhang, Ruicong Li, Jiajun Zhu, Jiaqi Yang, Yanan Zhang, Zhibo Cao, Wenxin Ji, Dongchao Zhang, Yumin |
| Author_xml | – sequence: 1 givenname: Jiajun surname: Li fullname: Li, Jiajun organization: Zhengzhou Research Institute, Harbin Institute of Technology , China – sequence: 2 givenname: Dongchao surname: Ji fullname: Ji, Dongchao organization: National Key Laboratory of Science and Technology on Advanced Composites in Special Environments, Harbin Institute of Technology , China – sequence: 3 givenname: Zhibo surname: Zhang fullname: Zhang, Zhibo organization: Zhengzhou Research Institute, Harbin Institute of Technology , China – sequence: 4 givenname: Yanan surname: Yang fullname: Yang, Yanan organization: Key Laboratory of Photoelectronic/Electrophotonic Conversion Materials and Key Laboratory of Cluster Science of Ministry of Education, School of Chemistry and Chemical Engineering, Beijing Institute of Technology , China – sequence: 5 givenname: Ruicong surname: Zhang fullname: Zhang, Ruicong organization: National Key Laboratory of Science and Technology on Advanced Composites in Special Environments, Harbin Institute of Technology , China – sequence: 6 givenname: Tianyu surname: Wang fullname: Wang, Tianyu organization: School of Energy Science & Engineering, Harbin Institute of Technology , China – sequence: 7 givenname: Yumin surname: Zhang fullname: Zhang, Yumin organization: National Key Laboratory of Science and Technology on Advanced Composites in Special Environments, Harbin Institute of Technology , China – sequence: 8 givenname: Wenxin surname: Cao fullname: Cao, Wenxin organization: Zhengzhou Research Institute, Harbin Institute of Technology , China – sequence: 9 givenname: Jiaqi surname: Zhu fullname: Zhu, Jiaqi organization: Zhengzhou Research Institute, Harbin Institute of Technology , China |
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| Snippet | Polymer-liquid crystals (PLCs) are common materials for smart windows. However, PLC smart windows usually require high driving voltage to maintain... Polymer-liquid crystals(PLCs)are common materials for smart windows.However,PLC smart windows usually require high driving voltage to maintain transparency.We... |
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| Title | MWCNT Doped Reverse-Mode Polymer Network Liquid Crystals with Frequency Response Property |
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