Charge disproportionation induced exchange bias in La0.5Ca0.5FeO3-δ
We observed an exchange bias effect in La0.5Ca0.5FeO3 perovskite compound. The exchange bias is associated with the charge disproportionation transition from Fe4＋ions to Fe3＋and Fe5＋ions below 175 K. The competition between the ferromagnetic interaction of Fe3＋and Fe5＋ions and the antiferromagnetic...
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| Published in | Science China. Physics, mechanics & astronomy Vol. 56; no. 11; pp. 2085 - 2089 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Berlin/Heidelberg
Springer Berlin Heidelberg
01.11.2013
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1674-7348 1869-1927 |
| DOI | 10.1007/s11433-013-5252-9 |
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| Abstract | We observed an exchange bias effect in La0.5Ca0.5FeO3 perovskite compound. The exchange bias is associated with the charge disproportionation transition from Fe4＋ions to Fe3＋and Fe5＋ions below 175 K. The competition between the ferromagnetic interaction of Fe3＋and Fe5＋ions and the antiferromagnetic one of Fe3＋and Fe3＋ions results in a unidirectional anisotropy in the cluster-glass system. An antiferromagnetically interfacial exchange coupling constant Ji 1.95 meV at the cluster-glass region was yielded by fitting the cooling field-dependence of the exchange bias field. |
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| AbstractList | We observed an exchange bias effect in La
0.5
Ca
0.5
FeO
3-δ
perovskite compound. The exchange bias is associated with the charge disproportionation transition from Fe
4+
ions to Fe
3+
and Fe
5+
ions below 175 K. The competition between the ferromagnetic interaction of Fe
3+
and Fe
5+
ions and the antiferromagnetic one of Fe
3+
and Fe
3+
ions results in a unidirectional anisotropy in the cluster-glass system. An antiferromagnetically interfacial exchange coupling constant
J
i
≈−1.95 meV at the cluster-glass region was yielded by fitting the cooling field-dependence of the exchange bias field. We observed an exchange bias effect in La0.5Ca0.5FeO3-δ perovskite compound. The exchange bias is associated with the charge disproportionation transition from Fe4+ ions to Fe3+ and Fe5+ ions below 175 K. The competition between the ferromagnetic interaction of Fe3+ and Fe5+ ions and the antiferromagnetic one of Fe3+ and Fe3+ ions results in a unidirectional anisotropy in the cluster-glass system. An antiferromagnetically interfacial exchange coupling constant Ji≈−1.95 meV at the cluster-glass region was yielded by fitting the cooling field-dependence of the exchange bias field. We observed an exchange bias effect in La0.5Ca0.5FeO3 perovskite compound. The exchange bias is associated with the charge disproportionation transition from Fe4＋ions to Fe3＋and Fe5＋ions below 175 K. The competition between the ferromagnetic interaction of Fe3＋and Fe5＋ions and the antiferromagnetic one of Fe3＋and Fe3＋ions results in a unidirectional anisotropy in the cluster-glass system. An antiferromagnetically interfacial exchange coupling constant Ji 1.95 meV at the cluster-glass region was yielded by fitting the cooling field-dependence of the exchange bias field. |
| Author | LIANG YaQiong ZHANG XiangQun JIN JinLing ZHAN QingFeng CHENG ZhaoHua |
| AuthorAffiliation | Logistic School, Beijing Wuzi University, Beijing 101149, China State Key Laboratory of Magnetism, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China Key Laboratory of Magnetic Materials and Devices, Ningbo Institute of Material Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China |
| Author_xml | – sequence: 1 givenname: YaQiong surname: Liang fullname: Liang, YaQiong organization: Logistic School, Beijing Wuzi University, State Key Laboratory of Magnetism, Institute of Physics, Chinese Academy of Sciences – sequence: 2 givenname: XiangQun surname: Zhang fullname: Zhang, XiangQun organization: State Key Laboratory of Magnetism, Institute of Physics, Chinese Academy of Sciences – sequence: 3 givenname: JinLing surname: Jin fullname: Jin, JinLing organization: State Key Laboratory of Magnetism, Institute of Physics, Chinese Academy of Sciences – sequence: 4 givenname: QingFeng surname: Zhan fullname: Zhan, QingFeng organization: Key Laboratory of Magnetic Materials and Devices, Ningbo Institute of Material Technology and Engineering, Chinese Academy of Sciences – sequence: 5 givenname: ZhaoHua surname: Cheng fullname: Cheng, ZhaoHua email: zhcheng@aphy.iphy.ac.cn organization: State Key Laboratory of Magnetism, Institute of Physics, Chinese Academy of Sciences |
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| Cites_doi | 10.1103/PhysRev.102.1413 10.1038/nature01687 10.1103/PhysRevLett.79.1393 10.1103/PhysRevB.43.1297 10.1103/PhysRevB.77.144409 10.1103/PhysRevB.61.3103 10.1103/PhysRevB.43.6031 10.1063/1.2730737 10.1103/PhysRevLett.80.181 10.1063/1.125573 10.1103/PhysRevB.72.134416 10.1088/0953-8984/20/44/445209 10.1023/B:REAC.0000019446.25192.67 10.1103/PhysRevB.73.174419 10.1103/PhysRevB.69.214431 10.1103/PhysRevB.72.174422 10.1016/S0304-8853(98)00266-2 10.1016/0025-5408(81)90138-0 10.1016/0022-4596(84)90275-5 10.1038/nnano.2007.292 10.1103/PhysRevLett.76.4624 10.1109/TMAG.1982.1061996 10.1023/B:REAC.0000019448.50672.f7 |
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| Keywords | charge disproportionation exchange bias cluster glass |
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| Notes | 11-5000/N exchange bias; charge disproportionation; cluster glass We observed an exchange bias effect in La0.5Ca0.5FeO3 perovskite compound. The exchange bias is associated with the charge disproportionation transition from Fe4＋ions to Fe3＋and Fe5＋ions below 175 K. The competition between the ferromagnetic interaction of Fe3＋and Fe5＋ions and the antiferromagnetic one of Fe3＋and Fe3＋ions results in a unidirectional anisotropy in the cluster-glass system. An antiferromagnetically interfacial exchange coupling constant Ji 1.95 meV at the cluster-glass region was yielded by fitting the cooling field-dependence of the exchange bias field. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 |
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| Snippet | We observed an exchange bias effect in La0.5Ca0.5FeO3 perovskite compound. The exchange bias is associated with the charge disproportionation transition from... We observed an exchange bias effect in La 0.5 Ca 0.5 FeO 3-δ perovskite compound. The exchange bias is associated with the charge disproportionation transition... We observed an exchange bias effect in La0.5Ca0.5FeO3-δ perovskite compound. The exchange bias is associated with the charge disproportionation transition from... |
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| SubjectTerms | Anisotropy Antiferromagnetism Astronomy Bias Charge exchange Classical and Continuum Physics Clusters Disproportionation Ferric ions Ferromagnetism Ions Observations and Techniques Perovskites Physics Physics and Astronomy 交换偏置场 充电 各向异性 歧化 玻璃系统 耦合常数 钙钛矿化合物 铁磁相互作用 |
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| Title | Charge disproportionation induced exchange bias in La0.5Ca0.5FeO3-δ |
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