Femtosecond solvation dynamics of indium dimers inside superfluid helium nanodroplets
Indium dimers (In 2 ) solvated inside helium nanodroplets are studied with femtosecond photoelectron and photoion spectroscopy. The solvation dynamics triggered by photoexcitation of the In 2 include expansion of the solvation shell and dopant ejection from the droplet, which both proceed more slowl...
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| Published in | EPJ Web of conferences Vol. 205; p. 6005 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article Conference Proceeding |
| Language | English |
| Published |
Les Ulis
EDP Sciences
2019
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 2100-014X 2101-6275 2100-014X |
| DOI | 10.1051/epjconf/201920506005 |
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| Abstract | Indium dimers (In
2
) solvated inside helium nanodroplets are studied with femtosecond photoelectron and photoion spectroscopy. The solvation dynamics triggered by photoexcitation of the In
2
include expansion of the solvation shell and dopant ejection from the droplet, which both proceed more slowly than for In atoms. Oscillation of the solvation shell, in contrast, is similar to the case of In atoms. These processes are observed in combination with intrinsic dynamics of the molecule and set the time-frame for the dopant interaction with the quantum fluid environment. |
|---|---|
| AbstractList | Indium dimers (In2) solvated inside helium nanodroplets are studied with femtosecond photoelectron and photoion spectroscopy. The solvation dynamics triggered by photoexcitation of the In2 include expansion of the solvation shell and dopant ejection from the droplet, which both proceed more slowly than for In atoms. Oscillation of the solvation shell, in contrast, is similar to the case of In atoms. These processes are observed in combination with intrinsic dynamics of the molecule and set the time-frame for the dopant interaction with the quantum fluid environment. Indium dimers (In 2 ) solvated inside helium nanodroplets are studied with femtosecond photoelectron and photoion spectroscopy. The solvation dynamics triggered by photoexcitation of the In 2 include expansion of the solvation shell and dopant ejection from the droplet, which both proceed more slowly than for In atoms. Oscillation of the solvation shell, in contrast, is similar to the case of In atoms. These processes are observed in combination with intrinsic dynamics of the molecule and set the time-frame for the dopant interaction with the quantum fluid environment. |
| Author | Meyer, Miriam Koch, Markus Heim, Pascal Thaler, Bernhard |
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| Cites_doi | 10.1063/1.4906512 10.1080/0144235X.2015.1051353 10.1080/0144235X.2014.937188 10.1103/PhysRevLett.95.163401 10.1016/0301-0104(95)00404-1 |
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| DOI | 10.1051/epjconf/201920506005 |
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| Snippet | Indium dimers (In
2
) solvated inside helium nanodroplets are studied with femtosecond photoelectron and photoion spectroscopy. The solvation dynamics... Indium dimers (In2) solvated inside helium nanodroplets are studied with femtosecond photoelectron and photoion spectroscopy. The solvation dynamics triggered... |
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| SubjectTerms | Dimers Dopants Ejection Fluids Helium Indium Photoelectrons Photoexcitation Solvation Superfluidity |
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| Title | Femtosecond solvation dynamics of indium dimers inside superfluid helium nanodroplets |
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