Solvent Effects on Linear and Multi-branched Bithiazole-based Derivatives Fluorescence Studied by Steady-state and Time-resovled Spectroscopy

Steady-state absorption, emission, and time-resolved spectroscopy were utilized to study the dynamics of excited states of linear and multi-branched bithiazole derivatives in different solvents at room temperature. In the studied compounds, triphenylamine and bithiazole groups act as donor and accep...

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Published in	Russian Journal of Physical Chemistry A Vol. 95; no. 8; pp. 1641 - 1645
Main Authors	Shi, Fuwen, Ni, Minghao, Wang, Zhiquan, He, Nannan, Li, Xiang, Hua, Jianli, Li, Bo, Chen, Ye
Format	Journal Article
Language	English
Published	Moscow Pleiades Publishing 01.08.2021 Springer Nature B.V
Subjects	Charge transfer Chemical bonds Chemistry Chemistry and Materials Science Doppler effect Emission analysis Fluorescence Molecular structure Physical Chemistry Red shift Room temperature Solvent effect Solvents Spectroscopic analysis Spectrum analysis Steady state Structure of Matter and Quantum Chemistry time-resolved spectroscopy solvent effect ICT
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ISSN	0036-0244 1531-863X
DOI	10.1134/S0036024421080215

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Abstract	Steady-state absorption, emission, and time-resolved spectroscopy were utilized to study the dynamics of excited states of linear and multi-branched bithiazole derivatives in different solvents at room temperature. In the studied compounds, triphenylamine and bithiazole groups act as donor and acceptor, respectively. BTZ-I and II have similar linear molecular structures, while BTZ-III and BTZ-IV have multi-branched structures. The difference is that the donor and acceptor units are connected by a single bond or a triple bond, respectively. With increase in solvent polarity, the fluorescence spectra exhibit a red shift and the fluorescence lifetime increases. Our results suggest there is intra-molecular charge transfer (ICT) processes in these four samples.
AbstractList	Steady-state absorption, emission, and time-resolved spectroscopy were utilized to study the dynamics of excited states of linear and multi-branched bithiazole derivatives in different solvents at room temperature. In the studied compounds, triphenylamine and bithiazole groups act as donor and acceptor, respectively. BTZ-I and II have similar linear molecular structures, while BTZ-III and BTZ-IV have multi-branched structures. The difference is that the donor and acceptor units are connected by a single bond or a triple bond, respectively. With increase in solvent polarity, the fluorescence spectra exhibit a red shift and the fluorescence lifetime increases. Our results suggest there is intra-molecular charge transfer (ICT) processes in these four samples.
Author	Li, Bo Ni, Minghao Wang, Zhiquan He, Nannan Hua, Jianli Li, Xiang Chen, Ye Shi, Fuwen
Author_xml	– sequence: 1 givenname: Fuwen surname: Shi fullname: Shi, Fuwen organization: Key Laboratory of Polar Materials and Devices (MOE), Department of Optoelectronics, East China Normal University – sequence: 2 givenname: Minghao surname: Ni fullname: Ni, Minghao organization: Key Laboratory of Polar Materials and Devices (MOE), Department of Optoelectronics, East China Normal University – sequence: 3 givenname: Zhiquan surname: Wang fullname: Wang, Zhiquan organization: Key Laboratory of Polar Materials and Devices (MOE), Department of Optoelectronics, East China Normal University – sequence: 4 givenname: Nannan surname: He fullname: He, Nannan organization: Key Laboratory for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology – sequence: 5 givenname: Xiang surname: Li fullname: Li, Xiang organization: Key Laboratory of Polar Materials and Devices (MOE), Department of Optoelectronics, East China Normal University – sequence: 6 givenname: Jianli surname: Hua fullname: Hua, Jianli organization: Key Laboratory for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology – sequence: 7 givenname: Bo surname: Li fullname: Li, Bo email: bli@ee.ecnu.edu.cn organization: Key Laboratory of Polar Materials and Devices (MOE), Department of Optoelectronics, East China Normal University – sequence: 8 givenname: Ye surname: Chen fullname: Chen, Ye email: ychen@ee.ecnu.edu.cn organization: Key Laboratory of Polar Materials and Devices (MOE), Department of Optoelectronics, East China Normal University
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SubjectTerms	Charge transfer Chemical bonds Chemistry Chemistry and Materials Science Doppler effect Emission analysis Fluorescence Molecular structure Physical Chemistry Red shift Room temperature Solvent effect Solvents Spectroscopic analysis Spectrum analysis Steady state Structure of Matter and Quantum Chemistry
Title	Solvent Effects on Linear and Multi-branched Bithiazole-based Derivatives Fluorescence Studied by Steady-state and Time-resovled Spectroscopy
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