Surface conversion derived core-shell nanostructures of Co particles@RuCo alloy for superior hydrogen evolution in alkali and seawater
Hydrogen evolution reaction (HER) in alkali involves higher energy barriers and slow reaction kinetics due to involving water dissociation process. Catalysts with proper surface properties are highly needed to optimize the surface binding energy with reaction intermediates and enhance intrinsic cata...
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| Published in | Applied catalysis. B, Environmental Vol. 315; p. 121554 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.10.2022
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0926-3373 1873-3883 |
| DOI | 10.1016/j.apcatb.2022.121554 |
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| Abstract | Hydrogen evolution reaction (HER) in alkali involves higher energy barriers and slow reaction kinetics due to involving water dissociation process. Catalysts with proper surface properties are highly needed to optimize the surface binding energy with reaction intermediates and enhance intrinsic catalytic activity. Herein, we present an effective strategy to construct a self-standing catalyst with core-shell structure, which is composited of metallic Co nanoparticles coated by RuCo alloy layer with optimized surface properties. The Ru attracts electrons from Co and optimizes the surface electronic structure. Theoretical calculations demonstrate that the water dissociation barrier on the Co surface is decreased from 0.65 eV to 0.58 eV after alloying with Ru. Experimental results reveal that the synthesized Co@RuCo-3 features highly efficient catalytic activity together with good stability at large current densities for HER in alkali, as well as in alkaline seawater and pure seawater.
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•Present an effective strategy to improve alkaline HER performance of Co.•Controllable coating MOF layers on nanomaterials.•A self-standing catalyst with core-shell nanostructure is constructed.•Self-standing Co@RuCo exhibits good long-term stability (100 h) at 500 mA cm−2. |
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| AbstractList | Hydrogen evolution reaction (HER) in alkali involves higher energy barriers and slow reaction kinetics due to involving water dissociation process. Catalysts with proper surface properties are highly needed to optimize the surface binding energy with reaction intermediates and enhance intrinsic catalytic activity. Herein, we present an effective strategy to construct a self-standing catalyst with core-shell structure, which is composited of metallic Co nanoparticles coated by RuCo alloy layer with optimized surface properties. The Ru attracts electrons from Co and optimizes the surface electronic structure. Theoretical calculations demonstrate that the water dissociation barrier on the Co surface is decreased from 0.65 eV to 0.58 eV after alloying with Ru. Experimental results reveal that the synthesized Co@RuCo-3 features highly efficient catalytic activity together with good stability at large current densities for HER in alkali, as well as in alkaline seawater and pure seawater.
[Display omitted]
•Present an effective strategy to improve alkaline HER performance of Co.•Controllable coating MOF layers on nanomaterials.•A self-standing catalyst with core-shell nanostructure is constructed.•Self-standing Co@RuCo exhibits good long-term stability (100 h) at 500 mA cm−2. |
| ArticleNumber | 121554 |
| Author | Jun, Hyunwoo Han, Jeong Woo Lee, Ahryeon Lee, Jinwoo Jung, Hyeonjung Huang, Huawei Kim, Seongbeen Park, Cheol-Young Choi, Jaeryung |
| Author_xml | – sequence: 1 givenname: Huawei surname: Huang fullname: Huang, Huawei organization: Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-Ro, Yuseong-Gu, Daejeon 34141, Republic of Korea – sequence: 2 givenname: Hyeonjung surname: Jung fullname: Jung, Hyeonjung organization: Department of Chemical Engineering, Pohang University of Science and Technology (POSTECH), Pohang, Gyeongbuk 37673, Republic of Korea – sequence: 3 givenname: Cheol-Young surname: Park fullname: Park, Cheol-Young organization: Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-Ro, Yuseong-Gu, Daejeon 34141, Republic of Korea – sequence: 4 givenname: Seongbeen surname: Kim fullname: Kim, Seongbeen organization: Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-Ro, Yuseong-Gu, Daejeon 34141, Republic of Korea – sequence: 5 givenname: Ahryeon surname: Lee fullname: Lee, Ahryeon organization: Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-Ro, Yuseong-Gu, Daejeon 34141, Republic of Korea – sequence: 6 givenname: Hyunwoo surname: Jun fullname: Jun, Hyunwoo organization: Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-Ro, Yuseong-Gu, Daejeon 34141, Republic of Korea – sequence: 7 givenname: Jaeryung surname: Choi fullname: Choi, Jaeryung organization: Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-Ro, Yuseong-Gu, Daejeon 34141, Republic of Korea – sequence: 8 givenname: Jeong Woo surname: Han fullname: Han, Jeong Woo email: jwhan@postech.ac.kr organization: Department of Chemical Engineering, Pohang University of Science and Technology (POSTECH), Pohang, Gyeongbuk 37673, Republic of Korea – sequence: 9 givenname: Jinwoo surname: Lee fullname: Lee, Jinwoo email: jwlee1@kaist.ac.kr organization: Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-Ro, Yuseong-Gu, Daejeon 34141, Republic of Korea |
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| Keywords | Electrocatalysis Cobalt Core-shell Alloy Hydrogen evolution |
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