Evaluation of various properties of ribbons of Mg-9%Al-3%Ca-based anode material for magnesium batteries produced by single-roll rapid solidification

There is an urgent need to develop next-generation rechargeable batteries for a carbon-neutral society. In this context, our research team is focusing on magnesium, which is abundant in the earth's crust and inexpensive. Ribbons of Mg-9%Al-3%Ca, a magnesium alloy, were prepared as anode materia...

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Published inJournal of Japan Institute of Light Metals Vol. 74; no. 10; pp. 455 - 462
Main Authors TABATA, Hironobu, HAGA, Toshio, AIDA, Tetsuo, KIRIMOTO, Yuichi, KURIHARA, Hideki, SUZUKI, Mayumi, TSUKEDA, Tadayoshi
Format Journal Article
LanguageJapanese
Published Tokyo The Japan Institute of Light Metals 15.10.2024
Japan Science and Technology Agency
Subjects
Online AccessGet full text
ISSN0451-5994
0368-5306
1880-8018
1880-8018
2186-618X
DOI10.2464/jilm.74.455

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Abstract There is an urgent need to develop next-generation rechargeable batteries for a carbon-neutral society. In this context, our research team is focusing on magnesium, which is abundant in the earth's crust and inexpensive. Ribbons of Mg-9%Al-3%Ca, a magnesium alloy, were prepared as anode material for rechargeable batteries by a single-roll rapid solidification method. The fabricated ribbons were subjected to various manufacturing conditions, and various properties such as surface properties, microstructure, mechanical properties, and electrochemical activity of the fabricated ribbons were evaluated. As a result, it was found that a peripheral speed of 25 m/s and an injection pressure of 0.05 MPa or less were desirable to fabricate ribbons with good surface and mechanical properties. It was also confirmed that electrochemical activity contributes significantly to the orientation of magnesium and that production conditions with a peripheral velocity of 30 m/s or higher resulted in low electrochemical activity.
AbstractList There is an urgent need to develop next-generation rechargeable batteries for a carbon-neutral society. In this context, our research team is focusing on magnesium, which is abundant in the earth's crust and inexpensive. Ribbons of Mg-9%Al-3%Ca, a magnesium alloy, were prepared as anode material for rechargeable batteries by a single-roll rapid solidification method. The fabricated ribbons were subjected to various manufacturing conditions, and various properties such as surface properties, microstructure, mechanical properties, and electrochemical activity of the fabricated ribbons were evaluated. As a result, it was found that a peripheral speed of 25 m/s and an injection pressure of 0.05 MPa or less were desirable to fabricate ribbons with good surface and mechanical properties. It was also confirmed that electrochemical activity contributes significantly to the orientation of magnesium and that production conditions with a peripheral velocity of 30 m/s or higher resulted in low electrochemical activity.
ArticleNumber 741001
Author TABATA, Hironobu
KIRIMOTO, Yuichi
KURIHARA, Hideki
HAGA, Toshio
TSUKEDA, Tadayoshi
AIDA, Tetsuo
SUZUKI, Mayumi
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  fullname: HAGA, Toshio
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  fullname: AIDA, Tetsuo
  organization: Faculty of Sustainable Design Academic Assembly, University of Toyama
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  fullname: KIRIMOTO, Yuichi
  organization: Department of Nano and Functional Material Science Graduate School of Science and Engineering for Education, University of Toyama
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  fullname: KURIHARA, Hideki
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References_xml – reference: 24) Y. Kirimoto, K. Fuke, T. Tsukeda, T. Aida, Y. Nemoto, M. Ikeda, H. Tabata, H. Kurihara and M. Suzuki: J. Japan Inst. Light Metals, 73 (2023), 537-544.
– reference: 12) X. Chen, S. Wei, F. Tong, M. P. Taylor and P. Cao: Electrochim. Acta, 398 (2021), 139336.
– reference: 16) Y. Orikasa: Bulletin of the Ceram. Soc. of Japan, 56 (2021), 343-346.
– reference: 21) K. Fuke, T. Tsukeda, T. Aida, M. Ikeda, H. Tabata, H. Kurihara and M. Suzuki: Proc. The 142th Conf. Japan Inst. Light Metals, (2022), 118-119.
– reference: 1) T. Tsukeda, T. Nakagawa, M. Moriwaki, K. Kikura, R. Sakurae, T. Aida, H. Tabata, H. Kurihara and M. Suzuki: Mater. Trans., 63 (2022), 408-414.
– reference: 6) K. Yamazaki: J. Japan Inst. Light Metals, 72 (2022), 92-98.
– reference: 33) M. Matsumoto: Bull. Res. Inst. Miner. Dressin. Metall, Tohoku Univ., 47 (1991), 141-144.
– reference: 26) Y. Kirimoto, T. Tsukeda, T. Aida, Y. Nemoto, M. Ikeda, H. Tabata, H. Kurihara and M. Suzuki: Proc. The 144th Conf. Japan Inst. Light Metals, (2023), 209-210.
– reference: 25) Y. Kirimoto, T. Tsukeda, T. Aida, Y. Nemoto, M. Ikeda, H. Tabata, H. Kurihara and M. Suzuki: Proc. The 143th Conf. Japan Inst. Light Metals, (2022), 99-100.
– reference: 2) T. Tsukeda, M. Moriwaki, T. Nakagawa, T. Aida, H. Tabata, H. Kurihara and M. Suzuki: Journal of JSEM., 22 (2022), 15-19.
– reference: 10) H. Kurihara, M. Inamoto and H. Ogasa: Chem. Lett., 50 (2021), 1213.
– reference: 11) H. K. Tian, R. Jalem, M. Matsui, T. Mandai, H. Somekawa and Y. Tateyama: J. Mater. Chem., A, 9 (2021), 15207.
– reference: 3) T. Tsukeda, Y. Kirimoto, T. Aida, M. Ikeda, H. Tabata, H. Kurihara, M. Suzuki and Y. Nemoto: ALUTOPIA, 53 (2023), 12-20.
– reference: 19) S. Yagi and T. Ichitsubo: Bulletin of the Ceram. Soc. of Japan, 56 (2021), 355-358.
– reference: 22) M. Ikeda, H. Tabata, K. Fuke, T. Tsukeda, T. Aida, H. Kurihara and M. Suzuki: Proc. The 143th Conf. Japan Inst. Light Metals, (2022), 95-96.
– reference: 23) K. Fuke, T. Tsukeda, T. Aida, M. Ikeda, H. Tabata, H. Kurihara and M. Suzuki: Proc. The 144th Conf. Japan Inst. Light Metals, (2023), 199-200.
– reference: 17) H. Watanabe and H. Imai: Bulletin of the Ceram. Soc. of Japan, 56 (2021), 347-350.
– reference: 13) K. Kanamura: Bulletin of the Ceram. Soc. of Japan, 56 (2021), 326-330.
– reference: 18) H. Kobayashi: Bulletin of the Ceram. Soc. of Japan, 56 (2021), 351-354.
– reference: 30) H. Sakamoto, N. Okumura, Y. Inoue and T. Yamada: J. Japan Inst. Metals, 60 (1996), 870-877.
– reference: 32) K. Fuke, Y. Kirimoto, T. Tsukeda, T. Aida, H. Tabata, H. Kurihara and M. Suzuki: Proc. The 145 Conf. Japan Inst. Light Metals, (2023), 85-86.
– reference: 7) D. Aurbach, H. Gizbar, A. Schechter, O. Chusid, H. E. Gottlieb, Y. Gofer and I. Goldberg: J. Electrochem. Soc., 149 (2002), A115.
– reference: 31) M. Inoue, M. Iwai, K. Matuzawa, S. Kamado and Y. Kojima: J. Japan Inst. Light Metals, 48 (1998), 257-262.
– reference: 28) T. Haga and M. Motomura: J. Japan Inst. Light Metals, 40 (1990), 265-270.
– reference: 9) T. Mandai and H. Somekawa: Chem. Commun., 56 (2020), 12122.
– reference: 4) S. Fukui, T. Tsukeda, T. Aida, H. Tabata, H. Kurihara and M. Suzuki: J. Japan Inst. Light Metals, 74 (2024), 14-17.
– reference: 5) T. Tsukeda: J. Japan Inst. Light Metals, 74 (2024), 227-232.
– reference: 27) Y. Kirimoto, T. Tsukeda, T. Aida, Y. Nemoto, M. Ikeda, H. Tabata, H. Kurihara and M. Suzuki: Proc. The 145th Conf. Japan Inst. Light Metals, (2023), 83-84.
– reference: 15) Y. Idemoto and N. Ishida: Bulletin of the Ceram. Soc. of Japan, 56 (2021), 337-342.
– reference: 8) Y. Gofer, O. Chusid, H. Gizbar, Y. Viestfrid, H. E. Gottlieb and D. Aurbach: Electrochem. Solid-State Lett., 9 (2006), A257.
– reference: 20) M. Nakayama, K. Nakano and R. Kobayashi: Bulletin of the Ceram. Soc. of Japan, 56 (2021), 362-365.
– reference: 29) K. Takeshita and H. Naya: J. Japan Inst. Metals. 60 (1996), 163-168.
– reference: 14) K. Shimokawa, N. Okamoto and T. Ichitsubo: Bulletin of the Ceram. Soc. of Japan, 56 (2021), 331-336.
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Snippet There is an urgent need to develop next-generation rechargeable batteries for a carbon-neutral society. In this context, our research team is focusing on...
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SubjectTerms Aluminum
Anodes
Calcium
Electrode materials
Magnesium base alloys
magnesium rechargeable battery
manufacturing process
Mechanical properties
Rapid solidification
Rechargeable batteries
Ribbons
single roll rapidly solidification method
Surface properties
Title Evaluation of various properties of ribbons of Mg-9%Al-3%Ca-based anode material for magnesium batteries produced by single-roll rapid solidification
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