Carbon Dioxide Solubilities in Decanoic Acid-Based Hydrophobic Deep Eutectic Solvents

The solubility of CO2 in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the temperature range from 298 to 323 K and at CO2 pressures up to 2 MPa. The results are evaluated by comparing the solubility data with existing hy...

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Published inJournal of chemical and engineering data Vol. 63; no. 4; pp. 913 - 919
Main Authors Zubeir, Lawien F, van Osch, Dannie J. G. P, Rocha, Marisa A. A, Banat, Fawzi, Kroon, Maaike C
Format Journal Article
LanguageEnglish
Published United States American Chemical Society 12.04.2018
Online AccessGet full text
ISSN0021-9568
1520-5134
DOI10.1021/acs.jced.7b00534

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Abstract The solubility of CO2 in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the temperature range from 298 to 323 K and at CO2 pressures up to 2 MPa. The results are evaluated by comparing the solubility data with existing hydrophilic DESs and currently applied physical solvents and fluorinated ionic liquids. The DESs are prepared by mixing decanoic acid with a quaternary ammonium salt with different halide anions and alkyl chain lengths. The measured CO2 solubilities are similar to those found in renowned fluorinated ILs, while the heats of CO2 absorption are in the range of nonpolar solvents. The presented DESs show good potential to be used as CO2 capture agents.
AbstractList The solubility of CO2 in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the temperature range from 298 to 323 K and at CO2 pressures up to 2 MPa. The results are evaluated by comparing the solubility data with existing hydrophilic DESs and currently applied physical solvents and fluorinated ionic liquids. The DESs are prepared by mixing decanoic acid with a quaternary ammonium salt with different halide anions and alkyl chain lengths. The measured CO2 solubilities are similar to those found in renowned fluorinated ILs, while the heats of CO2 absorption are in the range of nonpolar solvents. The presented DESs show good potential to be used as CO2 capture agents.
The solubility of CO2 in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the temperature range from 298 to 323 K and at CO2 pressures up to 2 MPa. The results are evaluated by comparing the solubility data with existing hydrophilic DESs and currently applied physical solvents and fluorinated ionic liquids. The DESs are prepared by mixing decanoic acid with a quaternary ammonium salt with different halide anions and alkyl chain lengths. The measured CO2 solubilities are similar to those found in renowned fluorinated ILs, while the heats of CO2 absorption are in the range of nonpolar solvents. The presented DESs show good potential to be used as CO2 capture agents.The solubility of CO2 in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the temperature range from 298 to 323 K and at CO2 pressures up to 2 MPa. The results are evaluated by comparing the solubility data with existing hydrophilic DESs and currently applied physical solvents and fluorinated ionic liquids. The DESs are prepared by mixing decanoic acid with a quaternary ammonium salt with different halide anions and alkyl chain lengths. The measured CO2 solubilities are similar to those found in renowned fluorinated ILs, while the heats of CO2 absorption are in the range of nonpolar solvents. The presented DESs show good potential to be used as CO2 capture agents.
The solubility of CO 2 in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the temperature range from 298 to 323 K and at CO 2 pressures up to 2 MPa. The results are evaluated by comparing the solubility data with existing hydrophilic DESs and currently applied physical solvents and fluorinated ionic liquids. The DESs are prepared by mixing decanoic acid with a quaternary ammonium salt with different halide anions and alkyl chain lengths. The measured CO 2 solubilities are similar to those found in renowned fluorinated ILs, while the heats of CO 2 absorption are in the range of nonpolar solvents. The presented DESs show good potential to be used as CO 2 capture agents.
The solubility of CO in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the temperature range from 298 to 323 K and at CO pressures up to 2 MPa. The results are evaluated by comparing the solubility data with existing hydrophilic DESs and currently applied physical solvents and fluorinated ionic liquids. The DESs are prepared by mixing decanoic acid with a quaternary ammonium salt with different halide anions and alkyl chain lengths. The measured CO solubilities are similar to those found in renowned fluorinated ILs, while the heats of CO absorption are in the range of nonpolar solvents. The presented DESs show good potential to be used as CO capture agents.
Author van Osch, Dannie J. G. P
Banat, Fawzi
Rocha, Marisa A. A
Zubeir, Lawien F
Kroon, Maaike C
AuthorAffiliation Chemical Engineering Department
Department of Chemical Engineering and Chemistry and Institute for Complex Molecular Systems, Laboratory of Physical Chemistry
Department of Chemical Engineering and Chemistry, Separation Technology Group
AuthorAffiliation_xml – name: Chemical Engineering Department
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  givenname: Lawien F
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  surname: Zubeir
  fullname: Zubeir, Lawien F
  email: LawienF.Zubeir@gmail.com
– sequence: 2
  givenname: Dannie J. G. P
  surname: van Osch
  fullname: van Osch, Dannie J. G. P
– sequence: 3
  givenname: Marisa A. A
  surname: Rocha
  fullname: Rocha, Marisa A. A
– sequence: 4
  givenname: Fawzi
  orcidid: 0000-0002-7646-5918
  surname: Banat
  fullname: Banat, Fawzi
  organization: Chemical Engineering Department
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  givenname: Maaike C
  orcidid: 0000-0002-5985-986X
  surname: Kroon
  fullname: Kroon, Maaike C
  organization: Chemical Engineering Department
BackLink https://www.ncbi.nlm.nih.gov/pubmed/29977093$$D View this record in MEDLINE/PubMed
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Snippet The solubility of CO2 in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the...
The solubility of CO in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the...
The solubility of CO 2 in hydrophobic deep eutectic solvents (DESs) has been measured for the first time. Six different hydrophobic DESs are studied in the...
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Title Carbon Dioxide Solubilities in Decanoic Acid-Based Hydrophobic Deep Eutectic Solvents
URI http://dx.doi.org/10.1021/acs.jced.7b00534
https://www.ncbi.nlm.nih.gov/pubmed/29977093
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