Virtual Colorimetric Sensor Array: Single Ionic Liquid for Solvent Discrimination
There is a continuing need to develop high-performance sensors for monitoring organic solvents, primarily due to the environmental impact of such compounds. In this regard, colorimetric sensors have been a subject of intense research for such applications. Herein, we report a unique virtual colorime...
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| Published in | Analytical chemistry (Washington) Vol. 87; no. 8; pp. 4464 - 4471 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
21.04.2015
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0003-2700 1520-6882 1520-6882 |
| DOI | 10.1021/acs.analchem.5b00714 |
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| Abstract | There is a continuing need to develop high-performance sensors for monitoring organic solvents, primarily due to the environmental impact of such compounds. In this regard, colorimetric sensors have been a subject of intense research for such applications. Herein, we report a unique virtual colorimetric sensor array based on a single ionic liquid (IL) for accurate detection and identification of similar organic solvents and mixtures of such solvents. In this study, we employ eight alcohols and seven binary mixtures of ethanol and methanol as analytes to provide a stringent test for assessing the capabilities of this array. The UV–visible spectra of alcoholic solutions of the IL used in this study show two absorption bands. Interestingly, the ratio of absorbance for these two bands is found to be extremely sensitive to alcohol polarity. A virtual sensor array is created by using four different concentrations of IL sensor, which allowed identification of these analytes with 96.4–100% accuracy. Overall, this virtual sensor array is found to be very promising for discrimination of closely related organic solvents. |
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| AbstractList | There is a continuing need to develop high-performance sensors for monitoring organic solvents, primarily due to the environmental impact of such compounds. In this regard, colorimetric sensors have been a subject of intense research for such applications. Herein, we report a unique virtual colorimetric sensor array based on a single ionic liquid (IL) for accurate detection and identification of similar organic solvents and mixtures of such solvents. In this study, we employ eight alcohols and seven binary mixtures of ethanol and methanol as analytes to provide a stringent test for assessing the capabilities of this array. The UV-visible spectra of alcoholic solutions of the IL used in this study show two absorption bands. Interestingly, the ratio of absorbance for these two bands is found to be extremely sensitive to alcohol polarity. A virtual sensor array is created by using four different concentrations of IL sensor, which allowed identification of these analytes with 96.4-100% accuracy. Overall, this virtual sensor array is found to be very promising for discrimination of closely related organic solvents. There is a continuing need to develop high-performance sensors for monitoring organic solvents, primarily due to the environmental impact of such compounds. In this regard, colorimetric sensors have been a subject of intense research for such applications. Herein, we report a unique virtual colorimetric sensor array based on a single ionic liquid (IL) for accurate detection and identification of similar organic solvents and mixtures of such solvents. In this study, we employ eight alcohols and seven binary mixtures of ethanol and methanol as analytes to provide a stringent test for assessing the capabilities of this array. The UV-visible spectra of alcoholic solutions of the IL used in this study show two absorption bands. Interestingly, the ratio of absorbance for these two bands is found to be extremely sensitive to alcohol polarity. A virtual sensor array is created by using four different concentrations of IL sensor, which allowed identification of these analytes with 96.4-100% accuracy. Overall, this virtual sensor array is found to be very promising for discrimination of closely related organic solvents.There is a continuing need to develop high-performance sensors for monitoring organic solvents, primarily due to the environmental impact of such compounds. In this regard, colorimetric sensors have been a subject of intense research for such applications. Herein, we report a unique virtual colorimetric sensor array based on a single ionic liquid (IL) for accurate detection and identification of similar organic solvents and mixtures of such solvents. In this study, we employ eight alcohols and seven binary mixtures of ethanol and methanol as analytes to provide a stringent test for assessing the capabilities of this array. The UV-visible spectra of alcoholic solutions of the IL used in this study show two absorption bands. Interestingly, the ratio of absorbance for these two bands is found to be extremely sensitive to alcohol polarity. A virtual sensor array is created by using four different concentrations of IL sensor, which allowed identification of these analytes with 96.4-100% accuracy. Overall, this virtual sensor array is found to be very promising for discrimination of closely related organic solvents. |
| Author | Galpothdeniya, Waduge Indika S Regmi, Bishnu P de Rooy, Sergio L Warner, Isiah M Siraj, Noureen McCarter, Kevin S |
| AuthorAffiliation | Department of Chemistry Department of Experimental Statistics Louisiana State University |
| AuthorAffiliation_xml | – name: Department of Experimental Statistics – name: Department of Chemistry – name: Louisiana State University |
| Author_xml | – sequence: 1 givenname: Waduge Indika S surname: Galpothdeniya fullname: Galpothdeniya, Waduge Indika S – sequence: 2 givenname: Bishnu P surname: Regmi fullname: Regmi, Bishnu P – sequence: 3 givenname: Kevin S surname: McCarter fullname: McCarter, Kevin S – sequence: 4 givenname: Sergio L surname: de Rooy fullname: de Rooy, Sergio L – sequence: 5 givenname: Noureen surname: Siraj fullname: Siraj, Noureen – sequence: 6 givenname: Isiah M surname: Warner fullname: Warner, Isiah M email: iwarner@lsu.edu |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25822878$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | absorbance absorption Alcohol Alcohols Analytical chemistry Aqueous solutions Chemical compounds Colorimetry Environmental impact Ethanol Ethyl alcohol Ionic liquids methanol Methyl alcohol monitoring Organic solvents Sensor arrays Sensors Solvents |
| Title | Virtual Colorimetric Sensor Array: Single Ionic Liquid for Solvent Discrimination |
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