Biogeochemistry of landfill leachate plumes
Information on attenuation processes controlling pollutants in leachate-affected aquifers is culled from the literature. Emphasis is on xenobiotic organic compounds, heavy metals, inorganic macrocomponents, and dissolved organic matter. Most leachate contamination plumes are relatively narrow and do...
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| Published in | Applied geochemistry Vol. 16; no. 7-8; pp. 659 - 718 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier
01.06.2001
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0883-2927 |
| DOI | 10.1016/S0883-2927(00)00082-2 |
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| Abstract | Information on attenuation processes controlling pollutants in leachate-affected aquifers is culled from the literature. Emphasis is on xenobiotic organic compounds, heavy metals, inorganic macrocomponents, and dissolved organic matter. Most leachate contamination plumes are relatively narrow and do not in terms of width exceed the width of a landfill. The importance of redox zones in understanding pollutant behavior as leachate migrates away from a landfill is stressed. Dissolved organic carbon appears to serve as a substrate for microbial redox processes. Heavy metals do not pose a major pollution problem at landfills, partly due to strong attenuation by sorption and precipitation. |
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| AbstractList | Information on attenuation processes controlling pollutants in leachate-affected aquifers is culled from the literature. Emphasis is on xenobiotic organic compounds, heavy metals, inorganic macrocomponents, and dissolved organic matter. Most leachate contamination plumes are relatively narrow and do not in terms of width exceed the width of a landfill. The importance of redox zones in understanding pollutant behavior as leachate migrates away from a landfill is stressed. Dissolved organic carbon appears to serve as a substrate for microbial redox processes. Heavy metals do not pose a major pollution problem at landfills, partly due to strong attenuation by sorption and precipitation. The literature has been critically reviewed in order to assess the attenuation processes governing contaminants in leachate affected aquifers. Attenuation here refers to dilution, sorption, ion exchange, precipitation, redox reactions and degradation processes. With respect to contaminants, focus is on dissolved organic matter, xenobiotic organic compounds, inorganic macrocomponents as anions and cations, and heavy metals. Laboratory as well as field investigations are included. This review is an up-date of an earlier comprehensive review. The review shows that most leachate contamination plumes are relatively narrow and do not in terms of width exceed the width of the landfill. The concept of redox zones being present in the plume has been confirmed by the reported composition of the leachate contaminated groundwater at several landfills and constitutes an important framework for understanding the behavior of the contaminants in the plume as the leachate migrates away from the landfill. Diverse microbial communities have been identified in leachate plumes and are believed to be responsible for the redox processes. Dissolved organic C in the leachate, although it appears to be only slowly degradable when the volatile organic acids are gone, apparently acts as substrate for the microbial redox processes. Several xenobiotic organic compounds have been found to be degradable in leachate contaminated groundwater, but degradation rates under anaerobic redox conditions have only been determined in a few cases. Apparently, observations in actual plumes indicate more extensive degradation than has been documented in the laboratory. The behavior of cations in leachate plumes is strongly influenced by exchange with the sediment, although the sediment often is very coarse and sandy. Ammonium seems to be subject to anaerobic oxidation, but the mechanisms are not yet understood. Heavy metals do not seem to constitute a significant pollution problem at landfills, partly because the heavy metal concentrations in the leachate often are low, and partly because of strong attenuation by sorption and precipitation. Although complexation of heavy metals with dissolved organic matter is significant, the heavy metals are in most cases still strongly attenuated in leachate-polluted aquifers. The information available on attenuation processes has increased dramatically during the last 15 a, but the number of well-documented full scale leachate plumes are still few and primarily from sandy aquifers. Thus, the diversity of attenuation processes in leachate plumes is probably not yet fully understood. Apparently, the attenuation processes in leachate plumes may for many contaminants provide significant natural remediation, limiting the effects of the leachate on the groundwater to an area usually not exceeding 1000 m from the landfill. |
| Author | Kjeldsen, Peter Baun, Anders Heron, Gorm Christensen, Jette B Bjerg, Poul L Jensen, Dorthe L Albrechtsen, Hans-Jørgen Christensen, Thomas H |
| Author_xml | – sequence: 1 givenname: Thomas H surname: Christensen fullname: Christensen, Thomas H – sequence: 2 givenname: Peter surname: Kjeldsen fullname: Kjeldsen, Peter – sequence: 3 givenname: Poul L surname: Bjerg fullname: Bjerg, Poul L – sequence: 4 givenname: Dorthe L surname: Jensen fullname: Jensen, Dorthe L – sequence: 5 givenname: Jette B surname: Christensen fullname: Christensen, Jette B – sequence: 6 givenname: Anders surname: Baun fullname: Baun, Anders – sequence: 7 givenname: Hans-Jørgen surname: Albrechtsen fullname: Albrechtsen, Hans-Jørgen – sequence: 8 givenname: Gorm surname: Heron fullname: Heron, Gorm |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=1134380$$DView record in Pascal Francis |
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| CODEN | APPGEY |
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| Snippet | Information on attenuation processes controlling pollutants in leachate-affected aquifers is culled from the literature. Emphasis is on xenobiotic organic... The literature has been critically reviewed in order to assess the attenuation processes governing contaminants in leachate affected aquifers. Attenuation here... |
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| SubjectTerms | dissolved organic matter Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics Exact sciences and technology Geochemistry Pollution, environment geology Soil and rock geochemistry |
| Title | Biogeochemistry of landfill leachate plumes |
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