Single Atom Substitution for Marking and Motion Tracking of Individual Molecules by Scanning Tunneling Microscopy

We report on a simple way to mark and track individual molecules self-assembled on a surface by scanning tunneling microscopy. The tracer mechanism consists in a minimal one-atom chemical substitution. While this substitution leads to significant modifications in the STM signature of the molecules,...

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Published inJournal of physical chemistry. C Vol. 112; no. 36; pp. 14058 - 14063
Main Authors Schull, Guillaume, Ness, Hervé, Douillard, Ludovic, Fiorini-Debuisschert, Céline, Charra, Fabrice, Mathevet, Fabrice, Kreher, David, Attias, André-Jean
Format Journal Article
LanguageEnglish
Published American Chemical Society 11.09.2008
Subjects
C: Surfaces, Interfaces, Catalysis
Chemical Sciences
Engineering Sciences
Material chemistry
Optics
Photonic
Online AccessGet full text
ISSN1932-7447
1932-7455
DOI10.1021/jp8030013

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Abstract We report on a simple way to mark and track individual molecules self-assembled on a surface by scanning tunneling microscopy. The tracer mechanism consists in a minimal one-atom chemical substitution. While this substitution leads to significant modifications in the STM signature of the molecules, no substantial changes of the physics of self-assembling are observed when using the modified or unmodified molecular building blocks. This allows us to follow the intrinsic dynamical properties of the self-assembled molecular patterns.
AbstractList We report on a simple way to mark and track individual molecules self-assembled on a surface by scanning tunneling microscopy. The tracer mechanism consists in a minimal one-atom chemical substitution. While this substitution leads to significant modifications in the STM signature of the molecules, no substantial changes of the physics of self-assembling are observed when using the modified or unmodified molecular building blocks. This allows us to follow the intrinsic dynamical properties of the self-assembled molecular patterns.
Author Mathevet, Fabrice
Charra, Fabrice
Kreher, David
Schull, Guillaume
Fiorini-Debuisschert, Céline
Douillard, Ludovic
Ness, Hervé
Attias, André-Jean
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Notes (i) Synthesis routes yielding to the unmarked (benzene core TSB) and marked (pyridine core TSP) molecular building blocks. (ii) Full description of the first-principle calculations carried on. This material is available free of charge via the Internet at http://pub.acs.org.
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Snippet We report on a simple way to mark and track individual molecules self-assembled on a surface by scanning tunneling microscopy. The tracer mechanism consists in...
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Chemical Sciences
Engineering Sciences
Material chemistry
Optics
Photonic
Title Single Atom Substitution for Marking and Motion Tracking of Individual Molecules by Scanning Tunneling Microscopy
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