Photoswitchable Intramolecular Through-Space Magnetic Interaction
The interaction between two TEMPO spin centers connected to a photoswitchable overcrowded alkene changes from noncoupled (three-line EPR spectrum) in the trans state, where the two spin centers are separated by ∼22 Å, to strongly coupled (five-line EPR spectrum) in the cis state, where the separatio...
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| Published in | Journal of the American Chemical Society Vol. 133; no. 21; pp. 8162 - 8164 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
WASHINGTON
American Chemical Society
01.06.2011
Amer Chemical Soc |
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| Online Access | Get full text |
| ISSN | 0002-7863 1520-5126 1520-5126 |
| DOI | 10.1021/ja202882q |
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| Abstract | The interaction between two TEMPO spin centers connected to a photoswitchable overcrowded alkene changes from noncoupled (three-line EPR spectrum) in the trans state, where the two spin centers are separated by ∼22 Å, to strongly coupled (five-line EPR spectrum) in the cis state, where the separation is ∼7 Å, upon photoswitching. Importantly, the performance of the alkene switching unit is essentially unaffected by the spin centers. |
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| AbstractList | The interaction between two TEMPO spin centers connected to a photoswitchable overcrowded alkene changes from noncoupled (three-line EPR spectrum) in the trans state, where the two spin centers are separated by ∼22 Å, to strongly coupled (five-line EPR spectrum) in the cis state, where the separation is ∼7 Å, upon photoswitching. Importantly, the performance of the alkene switching unit is essentially unaffected by the spin centers. The interaction between two TEMPO spin centers connected to a photoswitchable overcrowded alkene changes from noncoupled (three-line EPR spectrum) in the trans state, where the two spin centers are separated by ∼22 Å, to strongly coupled (five-line EPR spectrum) in the cis state, where the separation is ∼7 Å, upon photoswitching. Importantly, the performance of the alkene switching unit is essentially unaffected by the spin centers.The interaction between two TEMPO spin centers connected to a photoswitchable overcrowded alkene changes from noncoupled (three-line EPR spectrum) in the trans state, where the two spin centers are separated by ∼22 Å, to strongly coupled (five-line EPR spectrum) in the cis state, where the separation is ∼7 Å, upon photoswitching. Importantly, the performance of the alkene switching unit is essentially unaffected by the spin centers. The interaction between two TEMPO spin centers connected to a photoswitchable overcrowded alkene changes from noncoupled (three-line EPR spectrum) in the trans state, where the two spin centers are separated by similar to 22 angstrom, to strongly coupled (five-line EPR spectrum) in the cis state, where the separation is similar to 7 angstrom, upon photoswitching. Importantly, the performance of the alkene switching unit is essentially unaffected by the spin centers. |
| Author | Browne, Wesley R Hou, Lili Wang, Jiaobing Feringa, Ben L |
| AuthorAffiliation | University of Groningen |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/21542643$$D View this record in MEDLINE/PubMed |
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| Title | Photoswitchable Intramolecular Through-Space Magnetic Interaction |
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