Promoting Oxygen Evolution Reactions through Introduction of Oxygen Vacancies to Benchmark NiFe–OOH Catalysts
Advanced electrocatalysts toward oxygen evolution reaction (OER) at high current density with low overpotential remain a significant challenge for electrochemical water splitting. Herein, NiFe-based catalysts with appropriate electronic conductivity and catalytic activity have been obtained through...
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| Published in | ACS energy letters Vol. 3; no. 7; pp. 1515 - 1520 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
American Chemical Society
13.07.2018
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| Online Access | Get full text |
| ISSN | 2380-8195 2380-8195 |
| DOI | 10.1021/acsenergylett.8b00696 |
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| Abstract | Advanced electrocatalysts toward oxygen evolution reaction (OER) at high current density with low overpotential remain a significant challenge for electrochemical water splitting. Herein, NiFe-based catalysts with appropriate electronic conductivity and catalytic activity have been obtained through introduction of oxygen vacancies by a facile and economic NaBH4 reduction approach. The combined density functional theory calculations, physical characterization, and electrochemical studies disclose that the reductive treatment creates a high amount of oxygen vacancies, high active sites, and a low energy barrier for OER. The oxygen vacancy-rich catalyst yields a more than 2-fold increased current density (from 100 to 240 mA cm–2) at a low overpotential of 270 mV, accompanied by good stability under OER conditions. The approach is also broadly applicable for NiFe compounds synthesized via different methods or substrates. |
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| AbstractList | Advanced electrocatalysts toward oxygen evolution reaction (OER) at high current density with low overpotential remain a significant challenge for electrochemical water splitting. Herein, NiFe-based catalysts with appropriate electronic conductivity and catalytic activity have been obtained through introduction of oxygen vacancies by a facile and economic NaBH4 reduction approach. The combined density functional theory calculations, physical characterization, and electrochemical studies disclose that the reductive treatment creates a high amount of oxygen vacancies, high active sites, and a low energy barrier for OER. The oxygen vacancy-rich catalyst yields a more than 2-fold increased current density (from 100 to 240 mA cm–2) at a low overpotential of 270 mV, accompanied by good stability under OER conditions. The approach is also broadly applicable for NiFe compounds synthesized via different methods or substrates. |
| Author | Asnavandi, Majid Yin, Yichun Zhao, Chuan Li, Yibing Sun, Chenghua |
| AuthorAffiliation | Faculty of Science, Engineering & Technology School of Chemistry, Faculty of Science Swinburne University of Technology School of Chemistry |
| AuthorAffiliation_xml | – name: Swinburne University of Technology – name: Faculty of Science, Engineering & Technology – name: School of Chemistry, Faculty of Science – name: School of Chemistry |
| Author_xml | – sequence: 1 givenname: Majid orcidid: 0000-0001-5442-7294 surname: Asnavandi fullname: Asnavandi, Majid organization: School of Chemistry – sequence: 2 givenname: Yichun surname: Yin fullname: Yin, Yichun organization: School of Chemistry, Faculty of Science – sequence: 3 givenname: Yibing orcidid: 0000-0002-1729-5963 surname: Li fullname: Li, Yibing organization: School of Chemistry – sequence: 4 givenname: Chenghua surname: Sun fullname: Sun, Chenghua email: chenghuasun@swin.edu.au organization: Swinburne University of Technology – sequence: 5 givenname: Chuan orcidid: 0000-0001-7007-5946 surname: Zhao fullname: Zhao, Chuan email: chuan.zhao@unsw.edu.au organization: School of Chemistry |
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| Snippet | Advanced electrocatalysts toward oxygen evolution reaction (OER) at high current density with low overpotential remain a significant challenge for... |
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| Title | Promoting Oxygen Evolution Reactions through Introduction of Oxygen Vacancies to Benchmark NiFe–OOH Catalysts |
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