Second-Harmonic Generation in Resonant Nonlinear Metasurfaces Based on Lithium Niobate

Lithium niobate is an excellent and widely used material for nonlinear frequency conversion due to its strong optical nonlinearity and broad transparency region. Here, we report the fabrication and experimental investigation of resonant nonlinear metasurfaces for second-harmonic generation based on...

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Published inNano letters Vol. 20; no. 12; pp. 8608 - 8614
Main Authors Fedotova, Anna, Younesi, Mohammadreza, Sautter, Jürgen, Vaskin, Aleksandr, Löchner, Franz J.F, Steinert, Michael, Geiss, Reinhard, Pertsch, Thomas, Staude, Isabelle, Setzpfandt, Frank
Format Journal Article
LanguageEnglish
Published American Chemical Society 09.12.2020
Subjects
Nonlinear metasurfaces
Mie-type resonances
Lithium niobate
Second-harmonic generation
Online AccessGet full text
ISSN1530-6984
1530-6992
1530-6992
DOI10.1021/acs.nanolett.0c03290

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Abstract Lithium niobate is an excellent and widely used material for nonlinear frequency conversion due to its strong optical nonlinearity and broad transparency region. Here, we report the fabrication and experimental investigation of resonant nonlinear metasurfaces for second-harmonic generation based on thin-film lithium niobate. In the fabricated metasurfaces, we observe pronounced Mie-type resonances leading to enhanced second-harmonic generation in the direction normal to the metasurface. We find the largest second-harmonic generation efficiency for the resonance dominated by the electric contributions because its specific field distribution enables the most efficient usage of the largest element of the lithium niobate nonlinear susceptibility tensor. This is confirmed by polarization-resolved second-harmonic measurements, where we study contributions from different elements of the nonlinear susceptibility tensor to the total second-harmonic signal. Our work facilitates establishing lithium niobate as a material for resonant nanophotonics.
AbstractList Lithium niobate is an excellent and widely used material for nonlinear frequency conversion due to its strong optical nonlinearity and broad transparency region. Here, we report the fabrication and experimental investigation of resonant nonlinear metasurfaces for second-harmonic generation based on thin-film lithium niobate. In the fabricated metasurfaces, we observe pronounced Mie-type resonances leading to enhanced second-harmonic generation in the direction normal to the metasurface. We find the largest second-harmonic generation efficiency for the resonance dominated by the electric contributions because its specific field distribution enables the most efficient usage of the largest element of the lithium niobate nonlinear susceptibility tensor. This is confirmed by polarization-resolved second-harmonic measurements, where we study contributions from different elements of the nonlinear susceptibility tensor to the total second-harmonic signal. Our work facilitates establishing lithium niobate as a material for resonant nanophotonics.Lithium niobate is an excellent and widely used material for nonlinear frequency conversion due to its strong optical nonlinearity and broad transparency region. Here, we report the fabrication and experimental investigation of resonant nonlinear metasurfaces for second-harmonic generation based on thin-film lithium niobate. In the fabricated metasurfaces, we observe pronounced Mie-type resonances leading to enhanced second-harmonic generation in the direction normal to the metasurface. We find the largest second-harmonic generation efficiency for the resonance dominated by the electric contributions because its specific field distribution enables the most efficient usage of the largest element of the lithium niobate nonlinear susceptibility tensor. This is confirmed by polarization-resolved second-harmonic measurements, where we study contributions from different elements of the nonlinear susceptibility tensor to the total second-harmonic signal. Our work facilitates establishing lithium niobate as a material for resonant nanophotonics.
Lithium niobate is an excellent and widely used material for nonlinear frequency conversion due to its strong optical nonlinearity and broad transparency region. Here, we report the fabrication and experimental investigation of resonant nonlinear metasurfaces for second-harmonic generation based on thin-film lithium niobate. In the fabricated metasurfaces, we observe pronounced Mie-type resonances leading to enhanced second-harmonic generation in the direction normal to the metasurface. We find the largest second-harmonic generation efficiency for the resonance dominated by the electric contributions because its specific field distribution enables the most efficient usage of the largest element of the lithium niobate nonlinear susceptibility tensor. This is confirmed by polarization-resolved second-harmonic measurements, where we study contributions from different elements of the nonlinear susceptibility tensor to the total second-harmonic signal. Our work facilitates establishing lithium niobate as a material for resonant nanophotonics.
Author Pertsch, Thomas
Fedotova, Anna
Sautter, Jürgen
Geiss, Reinhard
Vaskin, Aleksandr
Younesi, Mohammadreza
Löchner, Franz J.F
Steinert, Michael
Setzpfandt, Frank
Staude, Isabelle
AuthorAffiliation Institute of Applied Physics, Abbe Center of Photonics
Fraunhofer Institute of Applied Optics and Precision Engineering
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Keywords Nonlinear metasurfaces
Mie-type resonances
Lithium niobate
Second-harmonic generation
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Snippet Lithium niobate is an excellent and widely used material for nonlinear frequency conversion due to its strong optical nonlinearity and broad transparency...
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Title Second-Harmonic Generation in Resonant Nonlinear Metasurfaces Based on Lithium Niobate
URI http://dx.doi.org/10.1021/acs.nanolett.0c03290
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