Orbital-Selective High-Temperature Cooper Pairing Developed in the Two-Dimensional Limit
For multiband superconductors, the orbital multiplicity yields orbital differentiation in normal-state properties and can lead to orbital-selective spin-fluctuation Cooper pairing. The orbital-selective phenomenon has become increasingly pivotal in clarifying the pairing “enigma”, particularly for m...
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Published in | Nano letters Vol. 22; no. 8; pp. 3245 - 3251 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
Published |
United States
American Chemical Society
27.04.2022
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Subjects | |
Online Access | Get full text |
ISSN | 1530-6984 1530-6992 1530-6992 |
DOI | 10.1021/acs.nanolett.1c04863 |
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Abstract | For multiband superconductors, the orbital multiplicity yields orbital differentiation in normal-state properties and can lead to orbital-selective spin-fluctuation Cooper pairing. The orbital-selective phenomenon has become increasingly pivotal in clarifying the pairing “enigma”, particularly for multiband high-temperature superconductors. Meanwhile, in one-unit-cell (1-UC) FeSe/SrTiO3, since the standard electron–hole Fermi pocket nesting scenario is inapplicable, the actual pairing mechanism is subject to intense debate. Here, by measuring high-resolution Bogoliubov quasiparticle interference, we report observations of highly anisotropic magnetic Cooper pairing in 1-UC FeSe. Theoretically, it is important to incorporate orbitally selective effects of electronic correlations within a spin-fluctuation pairing calculation, where the d xy orbital becomes coherence-suppressed. The resulting pairing gap is compatible with the experimental findings, which suggests that high-T c Cooper pairing with orbital selectivity applies to 2D-limit 1-UC FeSe. Our findings imply the general existence of orbital selectivity in iron-based superconductors and the universal significance of electron correlations in high-T c superconductors. |
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AbstractList | For multiband superconductors, the orbital multiplicity yields orbital differentiation in normal-state properties and can lead to orbital-selective spin-fluctuation Cooper pairing. The orbital-selective phenomenon has become increasingly pivotal in clarifying the pairing “enigma”, particularly for multiband high-temperature superconductors. Meanwhile, in one-unit-cell (1-UC) FeSe/SrTiO3, since the standard electron–hole Fermi pocket nesting scenario is inapplicable, the actual pairing mechanism is subject to intense debate. Here, by measuring high-resolution Bogoliubov quasiparticle interference, we report observations of highly anisotropic magnetic Cooper pairing in 1-UC FeSe. Theoretically, it is important to incorporate orbitally selective effects of electronic correlations within a spin-fluctuation pairing calculation, where the d xy orbital becomes coherence-suppressed. The resulting pairing gap is compatible with the experimental findings, which suggests that high-T c Cooper pairing with orbital selectivity applies to 2D-limit 1-UC FeSe. Our findings imply the general existence of orbital selectivity in iron-based superconductors and the universal significance of electron correlations in high-T c superconductors. For multiband superconductors, the orbital multiplicity yields orbital differentiation in normal-state properties and can lead to orbital-selective spin-fluctuation Cooper pairing. The orbital-selective phenomenon has become increasingly pivotal in clarifying the pairing "enigma", particularly for multiband high-temperature superconductors. Meanwhile, in one-unit-cell (1-UC) FeSe/SrTiO3, since the standard electron-hole Fermi pocket nesting scenario is inapplicable, the actual pairing mechanism is subject to intense debate. Here, by measuring high-resolution Bogoliubov quasiparticle interference, we report observations of highly anisotropic magnetic Cooper pairing in 1-UC FeSe. Theoretically, it is important to incorporate orbitally selective effects of electronic correlations within a spin-fluctuation pairing calculation, where the dxy orbital becomes coherence-suppressed. The resulting pairing gap is compatible with the experimental findings, which suggests that high-Tc Cooper pairing with orbital selectivity applies to 2D-limit 1-UC FeSe. Our findings imply the general existence of orbital selectivity in iron-based superconductors and the universal significance of electron correlations in high-Tc superconductors.For multiband superconductors, the orbital multiplicity yields orbital differentiation in normal-state properties and can lead to orbital-selective spin-fluctuation Cooper pairing. The orbital-selective phenomenon has become increasingly pivotal in clarifying the pairing "enigma", particularly for multiband high-temperature superconductors. Meanwhile, in one-unit-cell (1-UC) FeSe/SrTiO3, since the standard electron-hole Fermi pocket nesting scenario is inapplicable, the actual pairing mechanism is subject to intense debate. Here, by measuring high-resolution Bogoliubov quasiparticle interference, we report observations of highly anisotropic magnetic Cooper pairing in 1-UC FeSe. Theoretically, it is important to incorporate orbitally selective effects of electronic correlations within a spin-fluctuation pairing calculation, where the dxy orbital becomes coherence-suppressed. The resulting pairing gap is compatible with the experimental findings, which suggests that high-Tc Cooper pairing with orbital selectivity applies to 2D-limit 1-UC FeSe. Our findings imply the general existence of orbital selectivity in iron-based superconductors and the universal significance of electron correlations in high-Tc superconductors. For multiband superconductors, the orbital multiplicity yields orbital differentiation in normal-state properties and can lead to orbital-selective spin-fluctuation Cooper pairing. The orbital-selective phenomenon has become increasingly pivotal in clarifying the pairing "enigma", particularly for multiband high-temperature superconductors. Meanwhile, in one-unit-cell (1-UC) FeSe/SrTiO , since the standard electron-hole Fermi pocket nesting scenario is inapplicable, the actual pairing mechanism is subject to intense debate. Here, by measuring high-resolution Bogoliubov quasiparticle interference, we report observations of highly anisotropic magnetic Cooper pairing in 1-UC FeSe. Theoretically, it is important to incorporate orbitally selective effects of electronic correlations within a spin-fluctuation pairing calculation, where the d orbital becomes coherence-suppressed. The resulting pairing gap is compatible with the experimental findings, which suggests that high- Cooper pairing with orbital selectivity applies to 2D-limit 1-UC FeSe. Our findings imply the general existence of orbital selectivity in iron-based superconductors and the universal significance of electron correlations in high- superconductors. Not provided. |
Author | Li, Yu Wang, Jian Andersen, Brian M Liu, Chaofei Hirschfeld, Peter Kreisel, Andreas Zhong, Shan |
AuthorAffiliation | International Center for Quantum Materials, School of Physics University of Florida Niels Bohr Institute Beijing Academy of Quantum Information Sciences Universität Leipzig University of Copenhagen CAS Center for Excellence in Topological Quantum Computation Institut für Theoretische Physik Department of Physics University of Chinese Academy of Sciences |
AuthorAffiliation_xml | – name: Institut für Theoretische Physik – name: Niels Bohr Institute – name: Beijing Academy of Quantum Information Sciences – name: University of Florida – name: CAS Center for Excellence in Topological Quantum Computation – name: Department of Physics – name: International Center for Quantum Materials, School of Physics – name: University of Copenhagen – name: University of Chinese Academy of Sciences – name: Universität Leipzig |
Author_xml | – sequence: 1 givenname: Chaofei surname: Liu fullname: Liu, Chaofei organization: International Center for Quantum Materials, School of Physics – sequence: 2 givenname: Andreas surname: Kreisel fullname: Kreisel, Andreas organization: Universität Leipzig – sequence: 3 givenname: Shan surname: Zhong fullname: Zhong, Shan organization: International Center for Quantum Materials, School of Physics – sequence: 4 givenname: Yu surname: Li fullname: Li, Yu organization: International Center for Quantum Materials, School of Physics – sequence: 5 givenname: Brian M surname: Andersen fullname: Andersen, Brian M organization: University of Copenhagen – sequence: 6 givenname: Peter surname: Hirschfeld fullname: Hirschfeld, Peter organization: University of Florida – sequence: 7 givenname: Jian orcidid: 0000-0002-7212-0904 surname: Wang fullname: Wang, Jian email: jianwangphysics@pku.edu.cn organization: Beijing Academy of Quantum Information Sciences |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35416679$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1978187$$D View this record in Osti.gov |
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Keywords | orbital selectivity Cooper pairing one-unit-cell FeSe/SrTiO3 self-energy Bogoliubov quasiparticle interference |
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Title | Orbital-Selective High-Temperature Cooper Pairing Developed in the Two-Dimensional Limit |
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