Migration behavior of minor and rare earth elements in acidic soils and its controlling factors
The present study examines the migration behavior of minor and rare earth elements(REEs) in acidic soils such as andosol, loam and red-yellow soil. Al normalized values calculated from analytical results clearly indicate that the mobility of Ca, Mg, Sr and REEs in loam and red-yellow soil is smaller...
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| Published in | Shigen-Chishitsu Vol. 55; no. 2; pp. 169 - 180 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English Japanese |
| Published |
The Society of Resource Geology
2005
資源地質学会 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0918-2454 2185-4033 |
| DOI | 10.11456/shigenchishitsu1992.55.169 |
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| Abstract | The present study examines the migration behavior of minor and rare earth elements(REEs) in acidic soils such as andosol, loam and red-yellow soil. Al normalized values calculated from analytical results clearly indicate that the mobility of Ca, Mg, Sr and REEs in loam and red-yellow soil is smaller than that in andosol. The difference in the mobility of these elements is considered to have been caused by the different soil constituent minerals. Especially, the mobility of the REEs depend greatly on the type of clay mineral in soil. In the red-yellow soil containing illite, smectite and vermiculite, the lower mobility of light REEs compared with heavy REEs is controlled by the adsorption by these secondary minerals. On the other hand, in the andosol containing allophone, the higher mobility of the light REEs is controlled by the adsorption by allophane. This may be related to different hydrated ionic radii of each REE. |
|---|---|
| AbstractList | The present study examines the migration behavior of minor and rare earth elements(REEs) in acidic soils such as andosol, loam and red-yellow soil. Al normalized values calculated from analytical results clearly indicate that the mobility of Ca, Mg, Sr and REEs in loam and red-yellow soil is smaller than that in andosol. The difference in the mobility of these elements is considered to have been caused by the different soil constituent minerals. Especially, the mobility of the REEs depend greatly on the type of clay mineral in soil. In the red-yellow soil containing illite, smectite and vermiculite, the lower mobility of light REEs compared with heavy REEs is controlled by the adsorption by these secondary minerals. On the other hand, in the andosol containing allophone, the higher mobility of the light REEs is controlled by the adsorption by allophane. This may be related to different hydrated ionic radii of each REE. |
| Author | KUBOTA, Ran OTANI, Haruhiro SHIKAZONO, Naotatsu |
| Author_FL | 大谷 晴啓 鹿園 直建 久保 田蘭 |
| Author_FL_xml | – sequence: 1 fullname: 大谷 晴啓 – sequence: 2 fullname: 鹿園 直建 – sequence: 3 fullname: 久保 田蘭 |
| Author_xml | – sequence: 1 fullname: OTANI, Haruhiro organization: Department of Applied Chemistry, Faculty of Science and Technology, Keio University – sequence: 1 fullname: SHIKAZONO, Naotatsu organization: Department of Applied Chemistry, Faculty of Science and Technology, Keio University – sequence: 1 fullname: KUBOTA, Ran organization: Department of Applied Chemistry, Faculty of Science and Technology, Keio University |
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| Copyright | The Society of Resource Geology |
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| DOI | 10.11456/shigenchishitsu1992.55.169 |
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| DocumentTitleAlternate | 酸性土壌中の微量・希土類元素の移行挙動とその支配要因 |
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| References | Berger, G., Claparols, C., Guy, C. and Daux, V. (1994) Dissolution rate of a basalt glass in silica-rich solutions: Implications for long-term alteration. Geochim. Cosmochim. Acta, 58, 4875-4886. Brookins, D. G. (1978) Retention of transuranic and actinide elements and bismuth at the Oklo natural reactor, Gabon: Application of Eh-pH diagrams. Chem. Geol., 23, 309-323. 木村進一・鹿園直建・野原昌人・岩井修平(1999)化学的風化に伴う微量・希土類元素の挙動―男鹿半島,女川層堆積岩の例―.応用地質,40,281-294. Koeppenkastrop, D. and De Carlo, E. H. (1992) Sorption of rare earth elements from seawater onto synthetic mineral particles: An experimental approach. Chem. Geol., 95, 251-263. 南條正巳(1989)土壌中での元素の化学変化―多量元素,微量元素.「土の化学」社団法人日本化学会,112-128. 鹿園直建・瀧野晶嗣(2002)玄武岩ガラスの長期溶解速度の推定.原子力バックエンド研究,8,171-178. Yusa, Y. and Yamakawa, M. (1991) Tono in-situ research facilities for studies of the geological environment. 29th IGC Field Trip, B 18, 145-153 丸茂克美(2003)鉱物を用いた地質汚染浄化 In:資源環境地質学―地球史と環境汚染を読む―.資源地質,393-398. 加藤芳郎(1996)新版地学辞典.地学団体研究会,1443p. 岡崎正規・佐藤幸夫(1989)水和酸化物.「土の化学」社団法人日本化学会,67-79. 永塚鎮男(1997)原色日本土壌生態図鑑(株)フジ・テクノシステム,218p. 岩生周一(1985)粘土の辞典.朝倉書店,504p. 鹿園直建・大谷晴啓(2003)黒ボク土中の重金属元素の移行挙動とその支配要因.資源地質,53,147-152. 吉田英一・湯佐泰久(1995)放射性核種の地層中での挙動―東濃ウラン鉱床における天然ウラン系列核種を例にして―.同位元素研究発表会特別講演要旨,206-209. Stumm, W. (1992) Chemistry of the Solid-Water Interface. Wiley-Interscience, New York, 428p. Emerson, S. R. and Huested, S. S. (1991) Ocean anoxia and the concentrations of molybdenum and vanadium in seawater. Mar. Chem., 34, 177-196. Kevin, H. J. and Klaus, J. S. (1995) Speciation of rare earth element neodymium in groundwaters of the Nevada Test Site and Yucca Mountain and implications for actinide solubility. Appl. Geochem., 10, 565-572. Stumm, W. and Morgan, J. J. (1997) Aquatic Chemistry(3rd. ed.)-Chemical Equilibria and Rates in Natural Waters-. Wiley-Interscience, 1040p. Langmuir, D. (1997) Aqueous Environmental Geochemistry. Prentice Hall Upper Saddle River, New Jersey, 600p. German, C. R. and Elderfield, H. (1990) Application of the Ce anomaly as a paleoredox indicator: The ground rules. Paleoceanography, 5, 823-833. Takahashi, Y. and Minai, Y. (2001) Role of complex formation with humic substances in the redistribution of trivalent rare earth elements and actinides. Water-Rock Interaction. Swets & Zeitlinger, Lisse, 1465-1469. Arculus, R. J., Gust, D. A. and Kushiro, I. (1991) Fuji and Hakone. National Geographic Research & Exploration, 7, 276-309. 久保寺秀夫(2003)多様な理化学性の土壌が混在する地域での土壌管理とペドロジー―沖縄本島のマージ土壌の乾燥に伴う硬化の問題を例にして―.ペドロジスト,47,41-45. 和田光史・吉田稔・岡島英夫・鍬塚昭三(1991)土壌の吸着現象―基礎と応用―.日本土壌肥料学会編,博友社,160p. Compton, J. S., White, R. A. and Smith, M. (2003) Rare earth element behavior in soils and salt pan sediments of a semiarid granitic terrain in the Western Cape, South Africa. Chem. Geol., 201, 239-255. Nesbitt, H. W. (1979) Mobility and fractionation of rare earth elements during weathering of a granodiorite. Nature, 279, 206-210. Hill, I. G., Worden, R. H. and Meighan, I. G. (2000) Yttrium: the immobility-mobility transition during basaltic weathering. Geology, 28, 923-926. 三枝正彦(1989)黒ボク土.「土の化学」社団法人日本化学会,148-154. Sverjensky, D. A. (1994) Zero-point-of-charge prediction from crystal chemistry and solvation theory. Geochim. Cosmochim. Acta, 58, 3123-3129. Young, G. M. and Nesbitt, H. W. (1998) Processes controlling the distribution of Ti and Al in weathering profiles, siliciclastic sediments and sedimentary rocks. Jour. Sed. Res., 68, 448-455. 国土庁土地局国土調査課(1993)土地分類図(神奈川県,沖縄県).財団法人日本地図センター. Deer, W. A., Howie, R. A. and Zussman, W. (1963) Rock-forming minerals. William Clowes and Sons, 371 p. 鹿園直建・大谷晴啓・木村進一(2003)高レベル放射性廃棄物地層処分の安全性評価のためのナチュラルアナログ研究―風化作用による元素の移行評価―.資源地質,53,201-206. Aiuppa, A., Allard, P., D'Alessandro. W., Michel, A., Parello, F., Treuil, M. and Valenza, M. (2000) Mobility and fluxes of major, minor and trace metals during basalt weathering and groundwater transport at Mt. Etna volcano (Sicily). Geochim. Cosmochim. Acta, 64, 1827-1841. 丸茂克美(1995)地球表層の微細非晶質物質とは何か.地質ニュース,496,11-18. 赤川史典・吉田英一・与語節生・山本鋼志(2004)花崗岩割れ目周辺の酸化還元反応と二次的物質移動現象―地質環境中汚染物質の移動と長期的固定に関する研究―.地質雑,110,671-685. 松井健・永塚鎮男(1996)新版地学辞典.地学団体研究会,1443p. Winchester, J. A. and Floyd, P. A. (1977) Geochemical discimination of different magma series and their differentiation products using immobile elements. Chem. Geol., 20, 325-343. 古川博恭・黒田登美雄(1994)新しい石灰岩と古い石灰岩からなる沖縄島の地形,地質について―南部の[地下ダム]と,本部七不思議の1つ[塩川の湧水]―.土地分類技術資料・土地分類基本調査現地検討会資料―亜熱帯の地形,地質,土壌,土地利用―,11,20-49. Ohta, A. and Kawabe, I. (2001) REE (III) adsorption onto Mn dioxide (d-MnO2) and Fe oxyhydroxide: Ce (III) oxidation by d-MnO2. Geochim. Cosmochim. Acta, 65, 695-703. |
| References_xml | – reference: 鹿園直建・瀧野晶嗣(2002)玄武岩ガラスの長期溶解速度の推定.原子力バックエンド研究,8,171-178. – reference: Berger, G., Claparols, C., Guy, C. and Daux, V. (1994) Dissolution rate of a basalt glass in silica-rich solutions: Implications for long-term alteration. Geochim. Cosmochim. Acta, 58, 4875-4886. – reference: 久保寺秀夫(2003)多様な理化学性の土壌が混在する地域での土壌管理とペドロジー―沖縄本島のマージ土壌の乾燥に伴う硬化の問題を例にして―.ペドロジスト,47,41-45. – reference: Yusa, Y. and Yamakawa, M. (1991) Tono in-situ research facilities for studies of the geological environment. 29th IGC Field Trip, B 18, 145-153 – reference: German, C. R. and Elderfield, H. (1990) Application of the Ce anomaly as a paleoredox indicator: The ground rules. Paleoceanography, 5, 823-833. – reference: Koeppenkastrop, D. and De Carlo, E. H. (1992) Sorption of rare earth elements from seawater onto synthetic mineral particles: An experimental approach. Chem. Geol., 95, 251-263. – reference: 永塚鎮男(1997)原色日本土壌生態図鑑(株)フジ・テクノシステム,218p. – reference: 鹿園直建・大谷晴啓・木村進一(2003)高レベル放射性廃棄物地層処分の安全性評価のためのナチュラルアナログ研究―風化作用による元素の移行評価―.資源地質,53,201-206. – reference: 吉田英一・湯佐泰久(1995)放射性核種の地層中での挙動―東濃ウラン鉱床における天然ウラン系列核種を例にして―.同位元素研究発表会特別講演要旨,206-209. – reference: 松井健・永塚鎮男(1996)新版地学辞典.地学団体研究会,1443p. – reference: Compton, J. S., White, R. A. and Smith, M. (2003) Rare earth element behavior in soils and salt pan sediments of a semiarid granitic terrain in the Western Cape, South Africa. Chem. Geol., 201, 239-255. – reference: Winchester, J. A. and Floyd, P. A. (1977) Geochemical discimination of different magma series and their differentiation products using immobile elements. Chem. Geol., 20, 325-343. – reference: Emerson, S. R. and Huested, S. S. (1991) Ocean anoxia and the concentrations of molybdenum and vanadium in seawater. Mar. Chem., 34, 177-196. – reference: 南條正巳(1989)土壌中での元素の化学変化―多量元素,微量元素.「土の化学」社団法人日本化学会,112-128. – reference: Aiuppa, A., Allard, P., D'Alessandro. W., Michel, A., Parello, F., Treuil, M. and Valenza, M. (2000) Mobility and fluxes of major, minor and trace metals during basalt weathering and groundwater transport at Mt. Etna volcano (Sicily). Geochim. Cosmochim. Acta, 64, 1827-1841. – reference: 木村進一・鹿園直建・野原昌人・岩井修平(1999)化学的風化に伴う微量・希土類元素の挙動―男鹿半島,女川層堆積岩の例―.応用地質,40,281-294. – reference: Nesbitt, H. W. (1979) Mobility and fractionation of rare earth elements during weathering of a granodiorite. Nature, 279, 206-210. – reference: Deer, W. A., Howie, R. A. and Zussman, W. (1963) Rock-forming minerals. William Clowes and Sons, 371 p. – reference: Young, G. M. and Nesbitt, H. W. (1998) Processes controlling the distribution of Ti and Al in weathering profiles, siliciclastic sediments and sedimentary rocks. Jour. Sed. Res., 68, 448-455. – reference: 丸茂克美(2003)鉱物を用いた地質汚染浄化 In:資源環境地質学―地球史と環境汚染を読む―.資源地質,393-398. – reference: Stumm, W. (1992) Chemistry of the Solid-Water Interface. Wiley-Interscience, New York, 428p. – reference: Brookins, D. G. (1978) Retention of transuranic and actinide elements and bismuth at the Oklo natural reactor, Gabon: Application of Eh-pH diagrams. Chem. Geol., 23, 309-323. – reference: 赤川史典・吉田英一・与語節生・山本鋼志(2004)花崗岩割れ目周辺の酸化還元反応と二次的物質移動現象―地質環境中汚染物質の移動と長期的固定に関する研究―.地質雑,110,671-685. – reference: Arculus, R. J., Gust, D. A. and Kushiro, I. (1991) Fuji and Hakone. National Geographic Research & Exploration, 7, 276-309. – reference: 古川博恭・黒田登美雄(1994)新しい石灰岩と古い石灰岩からなる沖縄島の地形,地質について―南部の[地下ダム]と,本部七不思議の1つ[塩川の湧水]―.土地分類技術資料・土地分類基本調査現地検討会資料―亜熱帯の地形,地質,土壌,土地利用―,11,20-49. – reference: 和田光史・吉田稔・岡島英夫・鍬塚昭三(1991)土壌の吸着現象―基礎と応用―.日本土壌肥料学会編,博友社,160p. – reference: 丸茂克美(1995)地球表層の微細非晶質物質とは何か.地質ニュース,496,11-18. – reference: Sverjensky, D. A. (1994) Zero-point-of-charge prediction from crystal chemistry and solvation theory. Geochim. Cosmochim. Acta, 58, 3123-3129. – reference: Takahashi, Y. and Minai, Y. (2001) Role of complex formation with humic substances in the redistribution of trivalent rare earth elements and actinides. Water-Rock Interaction. Swets & Zeitlinger, Lisse, 1465-1469. – reference: 加藤芳郎(1996)新版地学辞典.地学団体研究会,1443p. – reference: Ohta, A. and Kawabe, I. (2001) REE (III) adsorption onto Mn dioxide (d-MnO2) and Fe oxyhydroxide: Ce (III) oxidation by d-MnO2. Geochim. Cosmochim. Acta, 65, 695-703. – reference: 岩生周一(1985)粘土の辞典.朝倉書店,504p. – reference: Kevin, H. J. and Klaus, J. S. (1995) Speciation of rare earth element neodymium in groundwaters of the Nevada Test Site and Yucca Mountain and implications for actinide solubility. Appl. Geochem., 10, 565-572. – reference: 国土庁土地局国土調査課(1993)土地分類図(神奈川県,沖縄県).財団法人日本地図センター. – reference: 鹿園直建・大谷晴啓(2003)黒ボク土中の重金属元素の移行挙動とその支配要因.資源地質,53,147-152. – reference: Langmuir, D. (1997) Aqueous Environmental Geochemistry. Prentice Hall Upper Saddle River, New Jersey, 600p. – reference: Stumm, W. and Morgan, J. J. (1997) Aquatic Chemistry(3rd. ed.)-Chemical Equilibria and Rates in Natural Waters-. Wiley-Interscience, 1040p. – reference: Hill, I. G., Worden, R. H. and Meighan, I. G. (2000) Yttrium: the immobility-mobility transition during basaltic weathering. Geology, 28, 923-926. – reference: 三枝正彦(1989)黒ボク土.「土の化学」社団法人日本化学会,148-154. – reference: 岡崎正規・佐藤幸夫(1989)水和酸化物.「土の化学」社団法人日本化学会,67-79. |
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| SubjectTerms | adsorption andosol clay minerals elemental mobility minor elements rare earth elements red soil weathering |
| Title | Migration behavior of minor and rare earth elements in acidic soils and its controlling factors |
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