Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene
This thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd-Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD)....
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| Main Author | |
|---|---|
| Corporate Author | |
| Format | Electronic eBook |
| Language | English |
| Published |
Singapore :
Springer Singapore : Imprint: Springer,
2017.
|
| Series | Springer Theses, Recognizing Outstanding Ph.D. Research,
|
| Subjects | |
| Online Access | Full text |
| ISBN | 9789811007736 |
| ISSN | 2190-5053 |
| DOI | 10.1007/978-981-10-0773-6 |
| Physical Description | 1 online resource (XII, 141 p. 83 illus., 42 illus. in color.) |
Cover
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| 100 | 1 | |a Hou, Ruijun. |e author. | |
| 245 | 1 | 0 | |a Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene / |c by Ruijun Hou. |
| 264 | 1 | |a Singapore : |b Springer Singapore : |b Imprint: Springer, |c 2017. | |
| 300 | |a 1 online resource (XII, 141 p. 83 illus., 42 illus. in color.) | ||
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| 490 | 1 | |a Springer Theses, Recognizing Outstanding Ph.D. Research, |x 2190-5053 | |
| 505 | 0 | |a Introduction -- Experimental and Theoretical Methods -- Design of Pd-Ni Bimetallic Catalyst -- Effect of Oxide Supports on Pd-Ni Bimetallic Catalysts -- Replacing Precious Metals with Carbide Catalysts -- Liquid Phase Hydrogenation of Acetylene -- Conclusion. | |
| 506 | |a Plný text je dostupný pouze z IP adres počítačů Univerzity Tomáše Bati ve Zlíně nebo vzdáleným přístupem pro zaměstnance a studenty | ||
| 520 | |a This thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd-Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD). The excellent correlation between model surfaces and supported catalysts demonstrates the feasibility of designing effective bimetallic catalysts for selective hydrogenation reactions. The author also proposes a method for designing non-precious metal catalysts to replace precious metals. She modifies the process of selective hydrogenation of acetylene by coupling the selective adsorption to the selective hydrogenation in the liquid phase, as a result of which the ethylene selectivity is greatly improved and heat transfer is greatly enhanced. Lastly, by analyzing the mechanism of liquid-phase hydrogenation, the author proposes a multi-stage slurry bed reactor for industrial applications.<. | ||
| 650 | 0 | |a Chemistry. | |
| 650 | 0 | |a Organic chemistry. | |
| 650 | 0 | |a Chemistry, Physical and theoretical. | |
| 650 | 0 | |a Chemical engineering. | |
| 650 | 0 | |a Catalysis. | |
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| 655 | 9 | |a electronic books |2 eczenas | |
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| 776 | 0 | 8 | |i Printed edition: |z 9789811007729 |
| 830 | 0 | |a Springer Theses, Recognizing Outstanding Ph.D. Research, |x 2190-5053 | |
| 856 | 4 | 0 | |u https://proxy.k.utb.cz/login?url=http://dx.doi.org/10.1007/978-981-10-0773-6 |
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